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Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing

Zhao, Lucy ; Spiehl, Dieter ; Kohnen, Marion C. ; Ceolin, Marcelo ; Mikolei, Joanna J. ; Pardehkhorram, Raheleh ; Andrieu‐Brunsen, Annette (2024)
Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing.
In: Small : nano micro, 2024, 20 (28)
doi: 10.26083/tuprints-00028300
Artikel, Zweitveröffentlichung, Verlagsversion

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Kurzbeschreibung (Abstract)

Combinatorial sensing is especially important in the context of modern drug development to enable fast screening of large data sets. Mesoporous silica materials offer high surface area and a wide range of functionalization possibilities. By adding structural control, the combination of structural and functional control along all length scales opens a new pathway that permits larger amounts of analytes being tested simultaneously for complex sensing tasks. This study presents a fast and simple way to produce mesoporous silica in various shapes and sizes between 0.27–6 mm by using light‐induced sol‐gel chemistry and digital light processing (DLP). Shape‐selective functionalization of mesoporous silica is successfully carried out either after printing using organosilanes or in situ while printing through the use of functional mesopore template for the in situ functionalization approach. Shape‐selective adsorption of dyes is shown as a demonstrator toward shape selective screening of potential analytes.

Typ des Eintrags: Artikel
Erschienen: 2024
Autor(en): Zhao, Lucy ; Spiehl, Dieter ; Kohnen, Marion C. ; Ceolin, Marcelo ; Mikolei, Joanna J. ; Pardehkhorram, Raheleh ; Andrieu‐Brunsen, Annette
Art des Eintrags: Zweitveröffentlichung
Titel: Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
Sprache: Englisch
Publikationsjahr: 12 November 2024
Ort: Darmstadt
Publikationsdatum der Erstveröffentlichung: 11 Juli 2024
Ort der Erstveröffentlichung: Weinheim
Verlag: Wiley-VCH
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Small : nano micro
Jahrgang/Volume einer Zeitschrift: 20
(Heft-)Nummer: 28
Kollation: 9 Seiten
DOI: 10.26083/tuprints-00028300
URL / URN: https://tuprints.ulb.tu-darmstadt.de/28300
Zugehörige Links:
Herkunft: Zweitveröffentlichung DeepGreen
Kurzbeschreibung (Abstract):

Combinatorial sensing is especially important in the context of modern drug development to enable fast screening of large data sets. Mesoporous silica materials offer high surface area and a wide range of functionalization possibilities. By adding structural control, the combination of structural and functional control along all length scales opens a new pathway that permits larger amounts of analytes being tested simultaneously for complex sensing tasks. This study presents a fast and simple way to produce mesoporous silica in various shapes and sizes between 0.27–6 mm by using light‐induced sol‐gel chemistry and digital light processing (DLP). Shape‐selective functionalization of mesoporous silica is successfully carried out either after printing using organosilanes or in situ while printing through the use of functional mesopore template for the in situ functionalization approach. Shape‐selective adsorption of dyes is shown as a demonstrator toward shape selective screening of potential analytes.

Freie Schlagworte: digital light processing, in situ functionalization, light‐induced self‐assembly, mesoporous silica, printing, sol‐gel chemistry
Status: Verlagsversion
URN: urn:nbn:de:tuda-tuprints-283001
Zusätzliche Informationen:

This article also appears in: Celebrating Excellence in the Advanced Materials Family: Women in Materials Science

Sachgruppe der Dewey Dezimalklassifikatin (DDC): 500 Naturwissenschaften und Mathematik > 540 Chemie
Fachbereich(e)/-gebiet(e): 07 Fachbereich Chemie
07 Fachbereich Chemie > Ernst-Berl-Institut
07 Fachbereich Chemie > Ernst-Berl-Institut > Fachgebiet Makromolekulare Chemie
07 Fachbereich Chemie > Ernst-Berl-Institut > Fachgebiet Makromolekulare Chemie > Smart Membranes
Hinterlegungsdatum: 12 Nov 2024 13:18
Letzte Änderung: 13 Nov 2024 06:54
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