Zhao, Lucy ; Spiehl, Dieter ; Kohnen, Marion C. ; Ceolin, Marcelo ; Mikolei, Joanna J. ; Pardehkhorram, Raheleh ; Andrieu-Brunsen, Annette (2024)
Printing of in situ functionalized mesoporous silica with digital light processing for combinatorial sensing.
In: Small
doi: 10.1002/smll.202311121
Artikel, Bibliographie
Kurzbeschreibung (Abstract)
Abstract Combinatorial sensing is especially important in the context of modern drug development to enable fast screening of large data sets. Mesoporous silica materials offer high surface area and a wide range of functionalization possibilities. By adding structural control, the combination of structural and functional control along all length scales opens a new pathway that permits larger amounts of analytes being tested simultaneously for complex sensing tasks. This study presents a fast and simple way to produce mesoporous silica in various shapes and sizes between 0.27–6 mm by using light-induced sol-gel chemistry and digital light processing (DLP). Shape-selective functionalization of mesoporous silica is successfully carried out either after printing using organosilanes or in situ while printing through the use of functional mesopore template for the in situ functionalization approach. Shape-selective adsorption of dyes is shown as a demonstrator toward shape selective screening of potential analytes.
| Typ des Eintrags: | Artikel |
|---|---|
| Erschienen: | 2024 |
| Autor(en): | Zhao, Lucy ; Spiehl, Dieter ; Kohnen, Marion C. ; Ceolin, Marcelo ; Mikolei, Joanna J. ; Pardehkhorram, Raheleh ; Andrieu-Brunsen, Annette |
| Art des Eintrags: | Bibliographie |
| Titel: | Printing of in situ functionalized mesoporous silica with digital light processing for combinatorial sensing |
| Sprache: | Englisch |
| Publikationsjahr: | 2024 |
| Ort: | Weinheim |
| Verlag: | Wiley |
| Titel der Zeitschrift, Zeitung oder Schriftenreihe: | Small |
| Kollation: | 9 Seiten |
| DOI: | 10.1002/smll.202311121 |
| URL / URN: | https://onlinelibrary.wiley.com/doi/abs/10.1002/smll.2023111... |
| Kurzbeschreibung (Abstract): | Abstract Combinatorial sensing is especially important in the context of modern drug development to enable fast screening of large data sets. Mesoporous silica materials offer high surface area and a wide range of functionalization possibilities. By adding structural control, the combination of structural and functional control along all length scales opens a new pathway that permits larger amounts of analytes being tested simultaneously for complex sensing tasks. This study presents a fast and simple way to produce mesoporous silica in various shapes and sizes between 0.27–6 mm by using light-induced sol-gel chemistry and digital light processing (DLP). Shape-selective functionalization of mesoporous silica is successfully carried out either after printing using organosilanes or in situ while printing through the use of functional mesopore template for the in situ functionalization approach. Shape-selective adsorption of dyes is shown as a demonstrator toward shape selective screening of potential analytes. |
| Freie Schlagworte: | digital light processing, in situ functionalization, light-induced self-assembly, mesoporous silica, printing, sol-gel chemistry |
| ID-Nummer: | Artikel-ID: 2311121 |
| Zusätzliche Informationen: | Early View Article ; This article also appears in: Hot Topic: Mesoporous Materials |
| Fachbereich(e)/-gebiet(e): | 16 Fachbereich Maschinenbau 16 Fachbereich Maschinenbau > Institut für Druckmaschinen und Druckverfahren (IDD) 07 Fachbereich Chemie 07 Fachbereich Chemie > Ernst-Berl-Institut |
| Hinterlegungsdatum: | 16 Feb 2024 08:48 |
| Letzte Änderung: | 20 Feb 2024 06:25 |
| PPN: | 515627356 |
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