Stock, Sebastian ; Mirau, Luca ; Rutsch, Matthias ; Wismath, Sonja ; Kupnik, Mario ; Klitzing, Regine von ; Rahimzadeh, Amin (2024)
Ultrasound‐Induced Adsorption of Acousto‐Responsive Microgels at Water–Oil Interface.
In: Advanced Science, 2024, 11 (5)
doi: 10.26083/tuprints-00027104
Artikel, Zweitveröffentlichung, Verlagsversion
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Kurzbeschreibung (Abstract)
Ultrasonic mixing is a well‐established method to disperse and mix substances. However, the effects of ultrasound on dispersed soft particles as well as on their adsorption kinetics at interfaces remain unexplored. Ultrasound not only accelerates the movement of particles via acoustic streaming, but recent research indicates that it can also manipulate the interaction of soft particles with the surrounding liquid. In this study, it evaluates the adsorption kinetics of microgel at the water‐oil interface under the influence of ultrasound. It quantifies how acoustic streaming accelerates the reduction of interfacial tension. It uses high‐frequency and low‐amplitude ultrasound, which has no destructive effects. Furthermore, it discusses the ultrasound‐induced shrinking and thus interfacial rearrangement of the microgels, which plays a secondary but non‐negligible role on interfacial tension reduction. It shows that the decrease in interfacial tension due to the acoustic streaming is stronger for microgels with higher cross‐linker density. Moreover, it shows that ultrasound can induce a reversible decrease in interfacial tension due to the shrinkage of microgels at the interface. The presented results may lead to a better understanding in any field where ultrasonic waves meet soft particles, e.g., controlled destabilization in foams and emulsions or systems for drug release.
Typ des Eintrags: | Artikel |
---|---|
Erschienen: | 2024 |
Autor(en): | Stock, Sebastian ; Mirau, Luca ; Rutsch, Matthias ; Wismath, Sonja ; Kupnik, Mario ; Klitzing, Regine von ; Rahimzadeh, Amin |
Art des Eintrags: | Zweitveröffentlichung |
Titel: | Ultrasound‐Induced Adsorption of Acousto‐Responsive Microgels at Water–Oil Interface |
Sprache: | Englisch |
Publikationsjahr: | 19 Juni 2024 |
Ort: | Darmstadt |
Publikationsdatum der Erstveröffentlichung: | 2 Februar 2024 |
Ort der Erstveröffentlichung: | Weinheim |
Verlag: | Wiley-VCH |
Titel der Zeitschrift, Zeitung oder Schriftenreihe: | Advanced Science |
Jahrgang/Volume einer Zeitschrift: | 11 |
(Heft-)Nummer: | 5 |
Kollation: | 10 Seiten |
DOI: | 10.26083/tuprints-00027104 |
URL / URN: | https://tuprints.ulb.tu-darmstadt.de/27104 |
Zugehörige Links: | |
Herkunft: | Zweitveröffentlichung DeepGreen |
Kurzbeschreibung (Abstract): | Ultrasonic mixing is a well‐established method to disperse and mix substances. However, the effects of ultrasound on dispersed soft particles as well as on their adsorption kinetics at interfaces remain unexplored. Ultrasound not only accelerates the movement of particles via acoustic streaming, but recent research indicates that it can also manipulate the interaction of soft particles with the surrounding liquid. In this study, it evaluates the adsorption kinetics of microgel at the water‐oil interface under the influence of ultrasound. It quantifies how acoustic streaming accelerates the reduction of interfacial tension. It uses high‐frequency and low‐amplitude ultrasound, which has no destructive effects. Furthermore, it discusses the ultrasound‐induced shrinking and thus interfacial rearrangement of the microgels, which plays a secondary but non‐negligible role on interfacial tension reduction. It shows that the decrease in interfacial tension due to the acoustic streaming is stronger for microgels with higher cross‐linker density. Moreover, it shows that ultrasound can induce a reversible decrease in interfacial tension due to the shrinkage of microgels at the interface. The presented results may lead to a better understanding in any field where ultrasonic waves meet soft particles, e.g., controlled destabilization in foams and emulsions or systems for drug release. |
Freie Schlagworte: | interfacial tension, microgels, ultrasound, water–oil interface |
ID-Nummer: | Artikel-ID: 2305395 |
Status: | Verlagsversion |
URN: | urn:nbn:de:tuda-tuprints-271040 |
Sachgruppe der Dewey Dezimalklassifikatin (DDC): | 500 Naturwissenschaften und Mathematik > 530 Physik 600 Technik, Medizin, angewandte Wissenschaften > 621.3 Elektrotechnik, Elektronik |
Fachbereich(e)/-gebiet(e): | 18 Fachbereich Elektrotechnik und Informationstechnik 18 Fachbereich Elektrotechnik und Informationstechnik > Mess- und Sensortechnik 05 Fachbereich Physik 05 Fachbereich Physik > Institut für Physik Kondensierter Materie (IPKM) 05 Fachbereich Physik > Institut für Physik Kondensierter Materie (IPKM) > Soft Matter at Interfaces (SMI) |
Hinterlegungsdatum: | 19 Jun 2024 12:34 |
Letzte Änderung: | 20 Jun 2024 12:24 |
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- Ultrasound‐Induced Adsorption of Acousto‐Responsive Microgels at Water–Oil Interface. (deposited 19 Jun 2024 12:34) [Gegenwärtig angezeigt]
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