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Ultrasound‐Induced Adsorption of Acousto‐Responsive Microgels at Water–Oil Interface

Stock, Sebastian ; Mirau, Luca ; Rutsch, Matthias ; Wismath, Sonja ; Kupnik, Mario ; Klitzing, Regine von ; Rahimzadeh, Amin (2024)
Ultrasound‐Induced Adsorption of Acousto‐Responsive Microgels at Water–Oil Interface.
In: Advanced Science, 2024, 11 (5)
doi: 10.26083/tuprints-00027104
Artikel, Zweitveröffentlichung, Verlagsversion

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Kurzbeschreibung (Abstract)

Ultrasonic mixing is a well‐established method to disperse and mix substances. However, the effects of ultrasound on dispersed soft particles as well as on their adsorption kinetics at interfaces remain unexplored. Ultrasound not only accelerates the movement of particles via acoustic streaming, but recent research indicates that it can also manipulate the interaction of soft particles with the surrounding liquid. In this study, it evaluates the adsorption kinetics of microgel at the water‐oil interface under the influence of ultrasound. It quantifies how acoustic streaming accelerates the reduction of interfacial tension. It uses high‐frequency and low‐amplitude ultrasound, which has no destructive effects. Furthermore, it discusses the ultrasound‐induced shrinking and thus interfacial rearrangement of the microgels, which plays a secondary but non‐negligible role on interfacial tension reduction. It shows that the decrease in interfacial tension due to the acoustic streaming is stronger for microgels with higher cross‐linker density. Moreover, it shows that ultrasound can induce a reversible decrease in interfacial tension due to the shrinkage of microgels at the interface. The presented results may lead to a better understanding in any field where ultrasonic waves meet soft particles, e.g., controlled destabilization in foams and emulsions or systems for drug release.

Typ des Eintrags: Artikel
Erschienen: 2024
Autor(en): Stock, Sebastian ; Mirau, Luca ; Rutsch, Matthias ; Wismath, Sonja ; Kupnik, Mario ; Klitzing, Regine von ; Rahimzadeh, Amin
Art des Eintrags: Zweitveröffentlichung
Titel: Ultrasound‐Induced Adsorption of Acousto‐Responsive Microgels at Water–Oil Interface
Sprache: Englisch
Publikationsjahr: 19 Juni 2024
Ort: Darmstadt
Publikationsdatum der Erstveröffentlichung: 2 Februar 2024
Ort der Erstveröffentlichung: Weinheim
Verlag: Wiley-VCH
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Advanced Science
Jahrgang/Volume einer Zeitschrift: 11
(Heft-)Nummer: 5
Kollation: 10 Seiten
DOI: 10.26083/tuprints-00027104
URL / URN: https://tuprints.ulb.tu-darmstadt.de/27104
Zugehörige Links:
Herkunft: Zweitveröffentlichung DeepGreen
Kurzbeschreibung (Abstract):

Ultrasonic mixing is a well‐established method to disperse and mix substances. However, the effects of ultrasound on dispersed soft particles as well as on their adsorption kinetics at interfaces remain unexplored. Ultrasound not only accelerates the movement of particles via acoustic streaming, but recent research indicates that it can also manipulate the interaction of soft particles with the surrounding liquid. In this study, it evaluates the adsorption kinetics of microgel at the water‐oil interface under the influence of ultrasound. It quantifies how acoustic streaming accelerates the reduction of interfacial tension. It uses high‐frequency and low‐amplitude ultrasound, which has no destructive effects. Furthermore, it discusses the ultrasound‐induced shrinking and thus interfacial rearrangement of the microgels, which plays a secondary but non‐negligible role on interfacial tension reduction. It shows that the decrease in interfacial tension due to the acoustic streaming is stronger for microgels with higher cross‐linker density. Moreover, it shows that ultrasound can induce a reversible decrease in interfacial tension due to the shrinkage of microgels at the interface. The presented results may lead to a better understanding in any field where ultrasonic waves meet soft particles, e.g., controlled destabilization in foams and emulsions or systems for drug release.

Freie Schlagworte: interfacial tension, microgels, ultrasound, water–oil interface
ID-Nummer: Artikel-ID: 2305395
Status: Verlagsversion
URN: urn:nbn:de:tuda-tuprints-271040
Sachgruppe der Dewey Dezimalklassifikatin (DDC): 500 Naturwissenschaften und Mathematik > 530 Physik
600 Technik, Medizin, angewandte Wissenschaften > 621.3 Elektrotechnik, Elektronik
Fachbereich(e)/-gebiet(e): 18 Fachbereich Elektrotechnik und Informationstechnik
18 Fachbereich Elektrotechnik und Informationstechnik > Mess- und Sensortechnik
05 Fachbereich Physik
05 Fachbereich Physik > Institut für Physik Kondensierter Materie (IPKM)
05 Fachbereich Physik > Institut für Physik Kondensierter Materie (IPKM) > Soft Matter at Interfaces (SMI)
Hinterlegungsdatum: 19 Jun 2024 12:34
Letzte Änderung: 20 Jun 2024 12:24
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