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Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells

Bermúdez Agudelo, María Catalina ; Hampe, Manfred ; Reiber, Thorsten ; Abele, Eberhard (2023)
Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells.
In: Materials, 2020, 13 (9)
doi: 10.26083/tuprints-00016630
Artikel, Zweitveröffentlichung, Verlagsversion

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Kurzbeschreibung (Abstract)

A high-temperature proton exchange membrane fuel cell (HT-PEMFC) conventionally uses a planar design with carbon-based substrates as the gas diffusion layer (GDL) materials. However, the metal-based substrates allow for alternative designs. In this study, the applicability of porous thin-walled tubular elements made of 316L stainless steel as the anode GDL in a multi-layer tubular HT-PEMFC was investigated. The anode GDLs were fabricated via powder bed fusion using a laser beam (PBF-LB) process with defined porosities (14% and 16%). The morphology of the porous elements was compared using scanning electron microscopy (SEM) micrographs. The influence of the porosity on the fuel cell performance was evaluated through electrochemical characterization and a short-term stability test (45 h) in a commercial test station operated at 160 °C and ambient pressure, using hydrogen as the fuel and air as the oxidant. The results showed that the fuel cell manufactured upon the anode GDL with a porosity of 16% had a higher performance with a peak power density of 329.25 W/m² after 5 h of operation at 125.52 A/m² and a voltage degradation rate of 0.511 mV/h over the stability test period. Moreover, this work indicates that additive manufacturing could be a useful tool for further fuel cell development.

Typ des Eintrags: Artikel
Erschienen: 2023
Autor(en): Bermúdez Agudelo, María Catalina ; Hampe, Manfred ; Reiber, Thorsten ; Abele, Eberhard
Art des Eintrags: Zweitveröffentlichung
Titel: Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells
Sprache: Englisch
Publikationsjahr: 20 November 2023
Ort: Darmstadt
Publikationsdatum der Erstveröffentlichung: 2020
Ort der Erstveröffentlichung: Basel
Verlag: MDPI
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Materials
Jahrgang/Volume einer Zeitschrift: 13
(Heft-)Nummer: 9
Kollation: 12 Seiten
DOI: 10.26083/tuprints-00016630
URL / URN: https://tuprints.ulb.tu-darmstadt.de/16630
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Herkunft: Zweitveröffentlichung DeepGreen
Kurzbeschreibung (Abstract):

A high-temperature proton exchange membrane fuel cell (HT-PEMFC) conventionally uses a planar design with carbon-based substrates as the gas diffusion layer (GDL) materials. However, the metal-based substrates allow for alternative designs. In this study, the applicability of porous thin-walled tubular elements made of 316L stainless steel as the anode GDL in a multi-layer tubular HT-PEMFC was investigated. The anode GDLs were fabricated via powder bed fusion using a laser beam (PBF-LB) process with defined porosities (14% and 16%). The morphology of the porous elements was compared using scanning electron microscopy (SEM) micrographs. The influence of the porosity on the fuel cell performance was evaluated through electrochemical characterization and a short-term stability test (45 h) in a commercial test station operated at 160 °C and ambient pressure, using hydrogen as the fuel and air as the oxidant. The results showed that the fuel cell manufactured upon the anode GDL with a porosity of 16% had a higher performance with a peak power density of 329.25 W/m² after 5 h of operation at 125.52 A/m² and a voltage degradation rate of 0.511 mV/h over the stability test period. Moreover, this work indicates that additive manufacturing could be a useful tool for further fuel cell development.

Freie Schlagworte: additive manufacturing, gas diffusion layer (GDL), high-temperature proton exchange membrane fuel cell (HT-PEMFC), MEA preparation, porosity, powder bed fusion using a laser beam (PBF-LB), tubular design
Status: Verlagsversion
URN: urn:nbn:de:tuda-tuprints-166307
Zusätzliche Informationen:

This article belongs to the Section Energy Materials

Sachgruppe der Dewey Dezimalklassifikatin (DDC): 600 Technik, Medizin, angewandte Wissenschaften > 620 Ingenieurwissenschaften und Maschinenbau
Fachbereich(e)/-gebiet(e): 16 Fachbereich Maschinenbau
16 Fachbereich Maschinenbau > Institut für Produktionsmanagement und Werkzeugmaschinen (PTW)
16 Fachbereich Maschinenbau > Fachgebiet für Thermische Verfahrenstechnik (TVT)
16 Fachbereich Maschinenbau > Fachgebiet Nano- und Mikrofluidik (NMF)
Hinterlegungsdatum: 20 Nov 2023 14:51
Letzte Änderung: 21 Nov 2023 07:10
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