Bermúdez Agudelo, María Catalina ; Hampe, Manfred ; Reiber, Thorsten ; Abele, Eberhard (2023)
Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells.
In: Materials, 2020, 13 (9)
doi: 10.26083/tuprints-00016630
Artikel, Zweitveröffentlichung, Verlagsversion
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Kurzbeschreibung (Abstract)
A high-temperature proton exchange membrane fuel cell (HT-PEMFC) conventionally uses a planar design with carbon-based substrates as the gas diffusion layer (GDL) materials. However, the metal-based substrates allow for alternative designs. In this study, the applicability of porous thin-walled tubular elements made of 316L stainless steel as the anode GDL in a multi-layer tubular HT-PEMFC was investigated. The anode GDLs were fabricated via powder bed fusion using a laser beam (PBF-LB) process with defined porosities (14% and 16%). The morphology of the porous elements was compared using scanning electron microscopy (SEM) micrographs. The influence of the porosity on the fuel cell performance was evaluated through electrochemical characterization and a short-term stability test (45 h) in a commercial test station operated at 160 °C and ambient pressure, using hydrogen as the fuel and air as the oxidant. The results showed that the fuel cell manufactured upon the anode GDL with a porosity of 16% had a higher performance with a peak power density of 329.25 W/m² after 5 h of operation at 125.52 A/m² and a voltage degradation rate of 0.511 mV/h over the stability test period. Moreover, this work indicates that additive manufacturing could be a useful tool for further fuel cell development.
Typ des Eintrags: | Artikel |
---|---|
Erschienen: | 2023 |
Autor(en): | Bermúdez Agudelo, María Catalina ; Hampe, Manfred ; Reiber, Thorsten ; Abele, Eberhard |
Art des Eintrags: | Zweitveröffentlichung |
Titel: | Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells |
Sprache: | Englisch |
Publikationsjahr: | 20 November 2023 |
Ort: | Darmstadt |
Publikationsdatum der Erstveröffentlichung: | 2020 |
Ort der Erstveröffentlichung: | Basel |
Verlag: | MDPI |
Titel der Zeitschrift, Zeitung oder Schriftenreihe: | Materials |
Jahrgang/Volume einer Zeitschrift: | 13 |
(Heft-)Nummer: | 9 |
Kollation: | 12 Seiten |
DOI: | 10.26083/tuprints-00016630 |
URL / URN: | https://tuprints.ulb.tu-darmstadt.de/16630 |
Zugehörige Links: | |
Herkunft: | Zweitveröffentlichung DeepGreen |
Kurzbeschreibung (Abstract): | A high-temperature proton exchange membrane fuel cell (HT-PEMFC) conventionally uses a planar design with carbon-based substrates as the gas diffusion layer (GDL) materials. However, the metal-based substrates allow for alternative designs. In this study, the applicability of porous thin-walled tubular elements made of 316L stainless steel as the anode GDL in a multi-layer tubular HT-PEMFC was investigated. The anode GDLs were fabricated via powder bed fusion using a laser beam (PBF-LB) process with defined porosities (14% and 16%). The morphology of the porous elements was compared using scanning electron microscopy (SEM) micrographs. The influence of the porosity on the fuel cell performance was evaluated through electrochemical characterization and a short-term stability test (45 h) in a commercial test station operated at 160 °C and ambient pressure, using hydrogen as the fuel and air as the oxidant. The results showed that the fuel cell manufactured upon the anode GDL with a porosity of 16% had a higher performance with a peak power density of 329.25 W/m² after 5 h of operation at 125.52 A/m² and a voltage degradation rate of 0.511 mV/h over the stability test period. Moreover, this work indicates that additive manufacturing could be a useful tool for further fuel cell development. |
Freie Schlagworte: | additive manufacturing, gas diffusion layer (GDL), high-temperature proton exchange membrane fuel cell (HT-PEMFC), MEA preparation, porosity, powder bed fusion using a laser beam (PBF-LB), tubular design |
Status: | Verlagsversion |
URN: | urn:nbn:de:tuda-tuprints-166307 |
Zusätzliche Informationen: | This article belongs to the Section Energy Materials |
Sachgruppe der Dewey Dezimalklassifikatin (DDC): | 600 Technik, Medizin, angewandte Wissenschaften > 620 Ingenieurwissenschaften und Maschinenbau |
Fachbereich(e)/-gebiet(e): | 16 Fachbereich Maschinenbau 16 Fachbereich Maschinenbau > Institut für Produktionsmanagement und Werkzeugmaschinen (PTW) 16 Fachbereich Maschinenbau > Fachgebiet für Thermische Verfahrenstechnik (TVT) 16 Fachbereich Maschinenbau > Fachgebiet Nano- und Mikrofluidik (NMF) |
Hinterlegungsdatum: | 20 Nov 2023 14:51 |
Letzte Änderung: | 21 Nov 2023 07:10 |
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