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Correlation of Interface Structure with Magnetic Exchange in a Hard/Soft Magnetic Model Nanostructure

Sabet, S. ; Moradabadi, A. ; Gorji, S. ; Fawey, M. H. ; Hildebrandt, E. ; Radulov, I. ; Wang, D. ; Zhang, H. ; Kübel, C. ; Alff, L. (2019)
Correlation of Interface Structure with Magnetic Exchange in a Hard/Soft Magnetic Model Nanostructure.
In: Physical Review Applied, 11 (5)
doi: 10.1103/PhysRevApplied.11.054078
Artikel, Bibliographie

Kurzbeschreibung (Abstract)

Synthesis of hard/soft magnetically exchange-coupled heterostructures is one promising way to design energy-efficient rare-earth-free artificial magnetic materials for application as permanent magnets and in spintronics. As a model system, we experimentally investigate MnGa/FeCo bilayers and simulate their physical behavior in a combined density functional theory and micromagnetic approach. Using high-quality L10−Mn1.5Ga thin films with bulklike magnetic properties, we show that optimal coherent exchange coupling is obtained below a critical soft magnetic layer thickness that depends on the interface structure and composition. In particular, for atomically smooth and matched epitaxial interfaces of L10−Mn1.5Ga to a Co-terminated and Co-rich FeCo layer, coherent exchange coupling is observed for FeCo thicknesses below 2 nm. In optimized bilayers, the magnetic coercivity of MnGa (approximately 6 kOe) can be fully conserved while the overall saturation magnetization is increased beyond 1000emu/cm3. Our model correlates interface structure and magnetic exchange coupling, providing guidelines to engineer high-performance exchange-coupled heterostructures for permanent magnets or spintronic devices.

Typ des Eintrags: Artikel
Erschienen: 2019
Autor(en): Sabet, S. ; Moradabadi, A. ; Gorji, S. ; Fawey, M. H. ; Hildebrandt, E. ; Radulov, I. ; Wang, D. ; Zhang, H. ; Kübel, C. ; Alff, L.
Art des Eintrags: Bibliographie
Titel: Correlation of Interface Structure with Magnetic Exchange in a Hard/Soft Magnetic Model Nanostructure
Sprache: Englisch
Publikationsjahr: 29 Mai 2019
Verlag: American Physical Society (APS)
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Physical Review Applied
Jahrgang/Volume einer Zeitschrift: 11
(Heft-)Nummer: 5
DOI: 10.1103/PhysRevApplied.11.054078
URL / URN: https://doi.org/10.1103/PhysRevApplied.11.054078
Kurzbeschreibung (Abstract):

Synthesis of hard/soft magnetically exchange-coupled heterostructures is one promising way to design energy-efficient rare-earth-free artificial magnetic materials for application as permanent magnets and in spintronics. As a model system, we experimentally investigate MnGa/FeCo bilayers and simulate their physical behavior in a combined density functional theory and micromagnetic approach. Using high-quality L10−Mn1.5Ga thin films with bulklike magnetic properties, we show that optimal coherent exchange coupling is obtained below a critical soft magnetic layer thickness that depends on the interface structure and composition. In particular, for atomically smooth and matched epitaxial interfaces of L10−Mn1.5Ga to a Co-terminated and Co-rich FeCo layer, coherent exchange coupling is observed for FeCo thicknesses below 2 nm. In optimized bilayers, the magnetic coercivity of MnGa (approximately 6 kOe) can be fully conserved while the overall saturation magnetization is increased beyond 1000emu/cm3. Our model correlates interface structure and magnetic exchange coupling, providing guidelines to engineer high-performance exchange-coupled heterostructures for permanent magnets or spintronic devices.

Fachbereich(e)/-gebiet(e): 11 Fachbereich Material- und Geowissenschaften
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Fachgebiet Dünne Schichten
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > In-Situ Elektronenmikroskopie
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Fachgebiet Theorie magnetischer Materialien
Hinterlegungsdatum: 30 Mär 2020 09:13
Letzte Änderung: 13 Jan 2024 16:57
PPN:
Projekte: The authors acknowledge the LOEWE project RESPONSE funded by the Ministry of Higher Education, Research and the Arts (HMWK) and the high-performance computer center of Hessen (Lichtenberg).
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