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Epitaxial strain-engineered self-assembly of magnetic nanostructures in FeRh thin films

Witte, Ralf ; Kruk, Robert ; Molinari, Alan ; Wang, Di ; Schlabach, Sabine ; Brand, Richard A. ; Provenzano, Virgil ; Hahn, Horst (2016)
Epitaxial strain-engineered self-assembly of magnetic nanostructures in FeRh thin films.
In: Journal of Physics D: Applied Physics, 50 (2)
doi: 10.1088/1361-6463/50/2/025007
Artikel, Bibliographie

Kurzbeschreibung (Abstract)

In this paper we introduce an innovative bottom-\up approach for engineering self-\assembled magnetic nanostructures using epitaxial strain-\induced twinning and phase separation. X-\ray diffraction, Fe-57 Mossbauer spectroscopy, scanning tunneling microscopy, and transmission electron microscopy show that epitaxial films of a near-\equiatomic FeRh alloy respond to the applied epitaxial strain by laterally splitting into two structural phases on the nanometer length scale. Most importantly, these two structural phases differ with respect to their magnetic properties, one being paramagnetic and the other ferromagnetic, thus leading to the formation of a patterned magnetic nanostructure. It is argued that the phase separation directly results from the different strain-\dependence of the total energy of the two competing phases. This straightforward relation directly enables further tailoring and optimization of the nanostructures' properties.

Typ des Eintrags: Artikel
Erschienen: 2016
Autor(en): Witte, Ralf ; Kruk, Robert ; Molinari, Alan ; Wang, Di ; Schlabach, Sabine ; Brand, Richard A. ; Provenzano, Virgil ; Hahn, Horst
Art des Eintrags: Bibliographie
Titel: Epitaxial strain-engineered self-assembly of magnetic nanostructures in FeRh thin films
Sprache: Englisch
Publikationsjahr: 18 Januar 2016
Verlag: IOP Publishing, England
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Journal of Physics D: Applied Physics
Jahrgang/Volume einer Zeitschrift: 50
(Heft-)Nummer: 2
DOI: 10.1088/1361-6463/50/2/025007
Kurzbeschreibung (Abstract):

In this paper we introduce an innovative bottom-\up approach for engineering self-\assembled magnetic nanostructures using epitaxial strain-\induced twinning and phase separation. X-\ray diffraction, Fe-57 Mossbauer spectroscopy, scanning tunneling microscopy, and transmission electron microscopy show that epitaxial films of a near-\equiatomic FeRh alloy respond to the applied epitaxial strain by laterally splitting into two structural phases on the nanometer length scale. Most importantly, these two structural phases differ with respect to their magnetic properties, one being paramagnetic and the other ferromagnetic, thus leading to the formation of a patterned magnetic nanostructure. It is argued that the phase separation directly results from the different strain-\dependence of the total energy of the two competing phases. This straightforward relation directly enables further tailoring and optimization of the nanostructures' properties.

Freie Schlagworte: Magnetic nanostructure, self-assembly, strain-adaption, epitaxy, FeRh
Fachbereich(e)/-gebiet(e): 11 Fachbereich Material- und Geowissenschaften
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Gemeinschaftslabor Nanomaterialien
Hinterlegungsdatum: 27 Jul 2017 08:55
Letzte Änderung: 10 Mär 2022 14:01
PPN:
Sponsoren: The authors acknowledge funding by the Deutsche Forschungsgemeinschaft via HA1344/28-1.
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