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In situ Resonant Ultrasound Spectroscopy during irradiation of solids with relativistic heavy ions

Alencar, Igor ; Haussühl, Eiken ; Winkler, Björn ; Trautmann, Christina ; Schuster, Beatrice ; Severin, Daniel (2015)
In situ Resonant Ultrasound Spectroscopy during irradiation of solids with relativistic heavy ions.
In: Acta Materialia, 89
doi: 10.1016/j.actamat.2015.01.031
Artikel, Bibliographie

Kurzbeschreibung (Abstract)

Samples of steel, fused silica, CaF2, NaCl, and a (La,Eu)PO4 monazite ceramic were irradiated with Bi-209 (130 GeV) and U-238 (60 GeV) ions up to total fluences of 6 x 10(11) cm(-2). During beam exposure, resonant ultrasound spectra were recorded. No radiation-induced changes in the density and elastic stiffness coefficients were observed when comparing samples before and after irradiation. The irradiation caused fully reversible shifts of the resonance frequencies in all samples except NaCl, silica and monazite irradiated with U ions. These reversible shifts are due to a temperature increase during irradiation. The heating process was modelled quantitatively by an energy balance model. The average thickness traversed by the ions was estimated from geometrical considerations and the energy deposition was calculated with the SRIM software. The results from the model and these calculations are in good agreement. For NaCl, silica and monazite, a degradation of the samples was observed. Hence, in situ Resonant Ultrasound Spectroscopy can be used to monitor sample integrity and temperatures in harsh radiation environments. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.

Typ des Eintrags: Artikel
Erschienen: 2015
Autor(en): Alencar, Igor ; Haussühl, Eiken ; Winkler, Björn ; Trautmann, Christina ; Schuster, Beatrice ; Severin, Daniel
Art des Eintrags: Bibliographie
Titel: In situ Resonant Ultrasound Spectroscopy during irradiation of solids with relativistic heavy ions
Sprache: Englisch
Publikationsjahr: 1 Mai 2015
Verlag: Pergamon-Elsevier Science Ltd, Oxford, England
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Acta Materialia
Jahrgang/Volume einer Zeitschrift: 89
DOI: 10.1016/j.actamat.2015.01.031
Kurzbeschreibung (Abstract):

Samples of steel, fused silica, CaF2, NaCl, and a (La,Eu)PO4 monazite ceramic were irradiated with Bi-209 (130 GeV) and U-238 (60 GeV) ions up to total fluences of 6 x 10(11) cm(-2). During beam exposure, resonant ultrasound spectra were recorded. No radiation-induced changes in the density and elastic stiffness coefficients were observed when comparing samples before and after irradiation. The irradiation caused fully reversible shifts of the resonance frequencies in all samples except NaCl, silica and monazite irradiated with U ions. These reversible shifts are due to a temperature increase during irradiation. The heating process was modelled quantitatively by an energy balance model. The average thickness traversed by the ions was estimated from geometrical considerations and the energy deposition was calculated with the SRIM software. The results from the model and these calculations are in good agreement. For NaCl, silica and monazite, a degradation of the samples was observed. Hence, in situ Resonant Ultrasound Spectroscopy can be used to monitor sample integrity and temperatures in harsh radiation environments. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.

Freie Schlagworte: Radiation effets in solids, Resonant Ultrasound Spectroscopy, Swift ion damage, Elasticity
Fachbereich(e)/-gebiet(e): 11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Fachgebiet Ionenstrahlmodifizierte Materialien
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft
11 Fachbereich Material- und Geowissenschaften
Hinterlegungsdatum: 29 Feb 2016 13:49
Letzte Änderung: 29 Feb 2016 13:49
PPN:
Sponsoren: Financial support from German Federal Ministry of Education and Research (BMBF, projects 02NUK019E and 02NUK021F) is gratefully acknowledged., I.A. acknowledges Brazilian National Council for Scientific and Technological Development (CNPq, project 237039/2012-5) for a post-doctoral fellowship and E.H. wishes to thank German Research Foundation (DFG, project HA5137/3) for financial support.
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