Michel, M. ; Bour, J. ; Petersen, J. ; Arnoult, C. ; Ettingshausen, F. ; Roth, C. ; Ruch, D. (2010)
Atmospheric Plasma Deposition: A New Pathway in the Design of Conducting Polymer-Based Anodes for Hydrogen Fuel Cells.
In: Fuel Cells, 10 (6)
doi: 10.1002/fuce.201000050
Artikel, Bibliographie
Kurzbeschreibung (Abstract)
In this study, we explored thin films of nanofibrous functionalised conducting plasma polyaniline (pPANI) with platinum deposited by an atmospheric plasma deposition process for the potential design of anodes for hydrogen fuel cell applications. We observed that the incorporation of such a polymer, characterised by both electronic and ionic conductivity, associated with a catalyst in a 3D porous network, could lead to an increased probability of the three-phase contact to occur. In this context, aniline was mixed with functionalised platinum nanoparticles and used as the precursor. The role of these functionalised nanoparticles was not only to act as the catalyst for fuel cell purposes, but also as nucleation sites promoting the formation of the nanofibrous pPANI thin film during the plasma polymerisation. The morphology of the thin film was analysed by scanning electron microscopy and the efficiency, in terms of energy conversion, was assessed in a single fuel cell test bench.
| Typ des Eintrags: | Artikel |
|---|---|
| Erschienen: | 2010 |
| Autor(en): | Michel, M. ; Bour, J. ; Petersen, J. ; Arnoult, C. ; Ettingshausen, F. ; Roth, C. ; Ruch, D. |
| Art des Eintrags: | Bibliographie |
| Titel: | Atmospheric Plasma Deposition: A New Pathway in the Design of Conducting Polymer-Based Anodes for Hydrogen Fuel Cells |
| Sprache: | Englisch |
| Publikationsjahr: | Dezember 2010 |
| Verlag: | WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim |
| Titel der Zeitschrift, Zeitung oder Schriftenreihe: | Fuel Cells |
| Jahrgang/Volume einer Zeitschrift: | 10 |
| (Heft-)Nummer: | 6 |
| DOI: | 10.1002/fuce.201000050 |
| Kurzbeschreibung (Abstract): | In this study, we explored thin films of nanofibrous functionalised conducting plasma polyaniline (pPANI) with platinum deposited by an atmospheric plasma deposition process for the potential design of anodes for hydrogen fuel cell applications. We observed that the incorporation of such a polymer, characterised by both electronic and ionic conductivity, associated with a catalyst in a 3D porous network, could lead to an increased probability of the three-phase contact to occur. In this context, aniline was mixed with functionalised platinum nanoparticles and used as the precursor. The role of these functionalised nanoparticles was not only to act as the catalyst for fuel cell purposes, but also as nucleation sites promoting the formation of the nanofibrous pPANI thin film during the plasma polymerisation. The morphology of the thin film was analysed by scanning electron microscopy and the efficiency, in terms of energy conversion, was assessed in a single fuel cell test bench. |
| Freie Schlagworte: | Fuel Cell, Electrode, Plasma Polymer, Platinum Utilization, Polyaniline |
| Fachbereich(e)/-gebiet(e): | 11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Erneuerbare Energien 11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft 11 Fachbereich Material- und Geowissenschaften |
| Hinterlegungsdatum: | 22 Feb 2013 12:36 |
| Letzte Änderung: | 05 Mär 2013 10:05 |
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