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Electroluminescence from a single nanotube–molecule–nanotube junction

Marquardt, Christoph W. ; Grunder, Sergio ; Błaszczyk, Alfred ; Dehm, Simone ; Hennrich, Frank ; Löhneysen, Hilbert v. ; Mayor, Marcel ; Krupke, Ralph (2010)
Electroluminescence from a single nanotube–molecule–nanotube junction.
In: Nature Nanotechnology, 5 (12)
doi: 10.1038/nnano.2010.230
Artikel, Bibliographie

Kurzbeschreibung (Abstract)

The positioning of single molecules between nanoscale electrodes1, 2, 3, 4, 5, 6, 7, 8 has allowed their use as functional units in electronic devices. Although the electrical transport in such devices has been widely explored, optical measurements have been restricted to the observation of electroluminescence from nanocrystals and nanoclusters9, 10 and from molecules in a scanning tunnelling microscope setup11, 12. In this Letter, we report the observation of electroluminescence from the core of a rod-like molecule between two metallic single-walled carbon nanotube electrodes forming a rigid solid-state device. We also develop a simple model to explain the onset voltage for electroluminescence. These results suggest new characterization and functional possibilities, and demonstrate the potential of carbon nanotubes for use in molecular electronics.

Typ des Eintrags: Artikel
Erschienen: 2010
Autor(en): Marquardt, Christoph W. ; Grunder, Sergio ; Błaszczyk, Alfred ; Dehm, Simone ; Hennrich, Frank ; Löhneysen, Hilbert v. ; Mayor, Marcel ; Krupke, Ralph
Art des Eintrags: Bibliographie
Titel: Electroluminescence from a single nanotube–molecule–nanotube junction
Sprache: Englisch
Publikationsjahr: 28 November 2010
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Nature Nanotechnology
Jahrgang/Volume einer Zeitschrift: 5
(Heft-)Nummer: 12
DOI: 10.1038/nnano.2010.230
Kurzbeschreibung (Abstract):

The positioning of single molecules between nanoscale electrodes1, 2, 3, 4, 5, 6, 7, 8 has allowed their use as functional units in electronic devices. Although the electrical transport in such devices has been widely explored, optical measurements have been restricted to the observation of electroluminescence from nanocrystals and nanoclusters9, 10 and from molecules in a scanning tunnelling microscope setup11, 12. In this Letter, we report the observation of electroluminescence from the core of a rod-like molecule between two metallic single-walled carbon nanotube electrodes forming a rigid solid-state device. We also develop a simple model to explain the onset voltage for electroluminescence. These results suggest new characterization and functional possibilities, and demonstrate the potential of carbon nanotubes for use in molecular electronics.

Fachbereich(e)/-gebiet(e): 11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Fachgebiet Molekulare Nanostrukturen
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft
11 Fachbereich Material- und Geowissenschaften
Hinterlegungsdatum: 08 Nov 2011 11:34
Letzte Änderung: 05 Mär 2013 09:55
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