Brandner, Armin ; Lehnert, Kerstin ; Bienholz, Arne ; Lucas, Martin ; Claus, Peter (2009)
Production of Biomass-Derived Chemicals and Energy: Chemocatalytic Conversions of Glycerol.
In: Topics in Catalysis, 52 (3)
doi: 10.1007/s11244-008-9164-2
Artikel, Bibliographie
Kurzbeschreibung (Abstract)
The growing production of biodiesel as a renewable source-based fuel leads to an increased amount of glycerol. Thus, it is a favorable starting material to obtain highly functionalized products. From a variety of catalytic reactions three examples, namely glycerol oxidation, glycerol hydrogenolysis and aqueous-phase reforming, were chosen for detailed studies in our group. The experimental focus for the oxidation of glycerol was set on preparation and detailed examination of supported Pt-Bi catalysts in batch reactions as well as in continuous experiments using a trickle bed reactor. For aqueous-phase reforming of glycerol to hydrogen the addition of tin to supported platinum catalysts was investigated. Ruthenium and copper based catalysts could be successfully applied in the hydrogenolysis of glycerol to 1,2-propanediol.
| Typ des Eintrags: | Artikel |
|---|---|
| Erschienen: | 2009 |
| Autor(en): | Brandner, Armin ; Lehnert, Kerstin ; Bienholz, Arne ; Lucas, Martin ; Claus, Peter |
| Art des Eintrags: | Bibliographie |
| Titel: | Production of Biomass-Derived Chemicals and Energy: Chemocatalytic Conversions of Glycerol |
| Sprache: | Englisch |
| Publikationsjahr: | 3 März 2009 |
| Verlag: | Springer Netherlands |
| Titel der Zeitschrift, Zeitung oder Schriftenreihe: | Topics in Catalysis |
| Jahrgang/Volume einer Zeitschrift: | 52 |
| (Heft-)Nummer: | 3 |
| DOI: | 10.1007/s11244-008-9164-2 |
| Kurzbeschreibung (Abstract): | The growing production of biodiesel as a renewable source-based fuel leads to an increased amount of glycerol. Thus, it is a favorable starting material to obtain highly functionalized products. From a variety of catalytic reactions three examples, namely glycerol oxidation, glycerol hydrogenolysis and aqueous-phase reforming, were chosen for detailed studies in our group. The experimental focus for the oxidation of glycerol was set on preparation and detailed examination of supported Pt-Bi catalysts in batch reactions as well as in continuous experiments using a trickle bed reactor. For aqueous-phase reforming of glycerol to hydrogen the addition of tin to supported platinum catalysts was investigated. Ruthenium and copper based catalysts could be successfully applied in the hydrogenolysis of glycerol to 1,2-propanediol. |
| Freie Schlagworte: | Glycerol - Oxidation - Hydrogenolysis - Aqueous-phase reforming - Bimetallic catalyst - Trickle-bed reactor - Dihydroxyacetone - Glyceric acid - Propanediol - Hydrogen |
| Zusätzliche Informationen: | Published online: 7. Januar 2009 |
| Fachbereich(e)/-gebiet(e): | 07 Fachbereich Chemie 07 Fachbereich Chemie > Ernst-Berl-Institut > Fachgebiet Technische Chemie > Technische Chemie II 07 Fachbereich Chemie > Ernst-Berl-Institut > Fachgebiet Technische Chemie |
| Hinterlegungsdatum: | 20 Mär 2009 09:00 |
| Letzte Änderung: | 05 Mär 2013 09:18 |
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