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Magnetic flux dynamics and structural features in fluorinated HgBa₂CuO₄ as probed by ¹⁹F NMR

Gippius, Andrei Andreevich ; Morozova, E. N. ; Antipov, Evgeny V. ; Abakumov, A. M. ; Rozova, M. G. ; Lüders, Klaus ; Hoffmann, W. ; Buntkowsky, Gerd ; Klein, Oliver (2000)
Magnetic flux dynamics and structural features in fluorinated HgBa₂CuO₄ as probed by ¹⁹F NMR.
In: Physical Review B, 61 (21)
doi: 10.1103/PhysRevB.61.14370
Artikel, Bibliographie

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Kurzbeschreibung (Abstract)

¹⁹F NMR spectra and spin-lattice relaxation rates have been measured on two powder HgBa₂CuO₄Fₓ samples. The results combined with our neutron powder-diffraction data [A. M. Abakumov et al., Phys. Rev. Lett. 80, 385 (1998)] confirm that fluorine atoms can be successfully incorporated in the lattice of superconducting Hg-1201 phase in the nonstoichiometric O3 site. Partial occupation of another oxygen position by fluorine atoms reveals to be possible with the increase of F content. The temperature dependence of the ¹⁹F NMR linewidth reveals the crossover at 35 K in the magnetic-flux line structure between the low-temperature latticelike regime and high-temperature “melted” regime. For the 1/T₁ temperature dependence a maximum has been found at 65 K indicating the strong influence of magnetic-flux line motion on the ¹⁹F spin-lattice relaxation rate.

Typ des Eintrags: Artikel
Erschienen: 2000
Autor(en): Gippius, Andrei Andreevich ; Morozova, E. N. ; Antipov, Evgeny V. ; Abakumov, A. M. ; Rozova, M. G. ; Lüders, Klaus ; Hoffmann, W. ; Buntkowsky, Gerd ; Klein, Oliver
Art des Eintrags: Bibliographie
Titel: Magnetic flux dynamics and structural features in fluorinated HgBa₂CuO₄ as probed by ¹⁹F NMR
Sprache: Englisch
Publikationsjahr: 2000
Ort: Darmstadt
Verlag: American Physical Society
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Physical Review B
Jahrgang/Volume einer Zeitschrift: 61
(Heft-)Nummer: 21
DOI: 10.1103/PhysRevB.61.14370
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Kurzbeschreibung (Abstract):

¹⁹F NMR spectra and spin-lattice relaxation rates have been measured on two powder HgBa₂CuO₄Fₓ samples. The results combined with our neutron powder-diffraction data [A. M. Abakumov et al., Phys. Rev. Lett. 80, 385 (1998)] confirm that fluorine atoms can be successfully incorporated in the lattice of superconducting Hg-1201 phase in the nonstoichiometric O3 site. Partial occupation of another oxygen position by fluorine atoms reveals to be possible with the increase of F content. The temperature dependence of the ¹⁹F NMR linewidth reveals the crossover at 35 K in the magnetic-flux line structure between the low-temperature latticelike regime and high-temperature “melted” regime. For the 1/T₁ temperature dependence a maximum has been found at 65 K indicating the strong influence of magnetic-flux line motion on the ¹⁹F spin-lattice relaxation rate.

Sachgruppe der Dewey Dezimalklassifikatin (DDC): 500 Naturwissenschaften und Mathematik > 530 Physik
500 Naturwissenschaften und Mathematik > 540 Chemie
Fachbereich(e)/-gebiet(e): 07 Fachbereich Chemie
07 Fachbereich Chemie > Eduard Zintl-Institut
07 Fachbereich Chemie > Eduard Zintl-Institut > Fachgebiet Physikalische Chemie
Hinterlegungsdatum: 02 Aug 2024 12:54
Letzte Änderung: 02 Aug 2024 12:54
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