Schäfer, David ; Hankins, Kie ; Allion, Michelle ; Krewer, Ulrike ; Karcher, Franziska ; Derr, Laurin ; Schuster, Rolf ; Maibach, Julia ; Mück, Stefan ; Kramer, Dominik ; Mönig, Reiner ; Jeschull, Fabian ; Daboss, Sven ; Philipp, Tom ; Neusser, Gregor ; Romer, Jan ; Palanisamy, Krishnaveni ; Kranz, Christine ; Buchner, Florian ; Behm, R. Jürgen ; Ahmadian, Ali ; Kübel, Christian ; Mohammad, Irshad ; Samoson, Ago ; Witter, Raiker ; Smarsly, Bernd ; Rohnke, Marcus (2024)
Multiscale investigation of sodium‐ion battery anodes: analytical techniques and applications.
In: Advanced Energy Materials, 14 (15)
doi: 10.1002/aenm.202302830
Artikel, Bibliographie
Kurzbeschreibung (Abstract)
The anode/electrolyte interface behavior, and by extension, the overall cell performance of sodium-ion batteries is determined by a complex interaction of processes that occur at all components of the electrochemical cell across a wide range of size- and timescales. Single-scale studies may provide incomplete insights, as they cannot capture the full picture of this complex and intertwined behavior. Broad, multiscale studies are essential to elucidate these processes. Within this perspectives article, several analytical and theoretical techniques are introduced, and described how they can be combined to provide a more complete and comprehensive understanding of sodium-ion battery (SIB) performance throughout its lifetime, with a special focus on the interfaces of hard carbon anodes. These methods target various length- and time scales, ranging from micro to nano, from cell level to atomistic structures, and account for a broad spectrum of physical and (electro)chemical characteristics. Specifically, how mass spectrometric, microscopic, spectroscopic, electrochemical, thermodynamic, and physical methods can be employed to obtain the various types of information required to understand battery behavior will be explored. Ways are then discussed how these methods can be coupled together in order to elucidate the multiscale phenomena at the anode interface and develop a holistic understanding of their relationship to overall sodium-ion battery function.
Here, several analytical methods across multiple time and length scales are discussed, covering a wide range of physical and (electro)chemical properties. To fully grasp the complexity of sodium-ion battery anodes, integrated studies on the same battery system, ranging from the cellular level to the atomic level, are required.image
Typ des Eintrags: | Artikel |
---|---|
Erschienen: | 2024 |
Autor(en): | Schäfer, David ; Hankins, Kie ; Allion, Michelle ; Krewer, Ulrike ; Karcher, Franziska ; Derr, Laurin ; Schuster, Rolf ; Maibach, Julia ; Mück, Stefan ; Kramer, Dominik ; Mönig, Reiner ; Jeschull, Fabian ; Daboss, Sven ; Philipp, Tom ; Neusser, Gregor ; Romer, Jan ; Palanisamy, Krishnaveni ; Kranz, Christine ; Buchner, Florian ; Behm, R. Jürgen ; Ahmadian, Ali ; Kübel, Christian ; Mohammad, Irshad ; Samoson, Ago ; Witter, Raiker ; Smarsly, Bernd ; Rohnke, Marcus |
Art des Eintrags: | Bibliographie |
Titel: | Multiscale investigation of sodium‐ion battery anodes: analytical techniques and applications |
Sprache: | Englisch |
Publikationsjahr: | April 2024 |
Verlag: | Wiley-VCH |
Titel der Zeitschrift, Zeitung oder Schriftenreihe: | Advanced Energy Materials |
Jahrgang/Volume einer Zeitschrift: | 14 |
(Heft-)Nummer: | 15 |
DOI: | 10.1002/aenm.202302830 |
Kurzbeschreibung (Abstract): | The anode/electrolyte interface behavior, and by extension, the overall cell performance of sodium-ion batteries is determined by a complex interaction of processes that occur at all components of the electrochemical cell across a wide range of size- and timescales. Single-scale studies may provide incomplete insights, as they cannot capture the full picture of this complex and intertwined behavior. Broad, multiscale studies are essential to elucidate these processes. Within this perspectives article, several analytical and theoretical techniques are introduced, and described how they can be combined to provide a more complete and comprehensive understanding of sodium-ion battery (SIB) performance throughout its lifetime, with a special focus on the interfaces of hard carbon anodes. These methods target various length- and time scales, ranging from micro to nano, from cell level to atomistic structures, and account for a broad spectrum of physical and (electro)chemical characteristics. Specifically, how mass spectrometric, microscopic, spectroscopic, electrochemical, thermodynamic, and physical methods can be employed to obtain the various types of information required to understand battery behavior will be explored. Ways are then discussed how these methods can be coupled together in order to elucidate the multiscale phenomena at the anode interface and develop a holistic understanding of their relationship to overall sodium-ion battery function. Here, several analytical methods across multiple time and length scales are discussed, covering a wide range of physical and (electro)chemical properties. To fully grasp the complexity of sodium-ion battery anodes, integrated studies on the same battery system, ranging from the cellular level to the atomic level, are required.image |
Freie Schlagworte: | hard carbon, solid electrolyte interphase, multiscale, SEI, sodium-ion battery |
ID-Nummer: | Artikel-ID: 2302830 |
Fachbereich(e)/-gebiet(e): | 11 Fachbereich Material- und Geowissenschaften 11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft 11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > In-Situ Elektronenmikroskopie |
Hinterlegungsdatum: | 12 Jun 2024 09:37 |
Letzte Änderung: | 17 Jun 2024 09:05 |
PPN: | 519185366 |
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Suche nach Titel in: | TUfind oder in Google |
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