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Effect of temperature on dislocation-tuned dielectricity and piezoelectricity in single-crystal BaTiO3

Dietrich, Felix ; Ni, Fan ; Fulanović, Lovro ; Zhou, Xiandong ; Isaia, Daniel ; Groszewicz, Pedro B. ; Zhang, Chunlin ; Xu, Bai-Xiang ; Rödel, Jürgen ; Buntkowsky, Gerd ; Zhuo, Fangping (2024)
Effect of temperature on dislocation-tuned dielectricity and piezoelectricity in single-crystal BaTiO3.
In: Applied Physics Letters, 124
doi: 10.1063/5.0191394
Artikel, Bibliographie

Kurzbeschreibung (Abstract)

The pinning-controlled mobility of ferroelectric/ferroelastic domain walls is an important part of managing polarization switching and deter- mining the final properties of ferroelectric and piezoelectric materials. Here, we assess the impact of temperature on dislocation-induced domain wall pinning as well as on dislocation-tuned dielectric and piezoelectric response in barium titanate single crystals. Our solid-state nuclear magnetic resonance spectroscopy results indicate that the entire sample exclusively permits in-plane domains, with their distribution remaining insensitive to temperature changes below the Curie temperature (TC ). The domain wall pinning field monotonically decreases with increasing temperature up to TC , as evidenced by a combination of experimental observations and phase-field simulations. Our work high- lights the promising potential of dislocation engineering in controlling domain wall mobility within bulk ferroelectrics.

Typ des Eintrags: Artikel
Erschienen: 2024
Autor(en): Dietrich, Felix ; Ni, Fan ; Fulanović, Lovro ; Zhou, Xiandong ; Isaia, Daniel ; Groszewicz, Pedro B. ; Zhang, Chunlin ; Xu, Bai-Xiang ; Rödel, Jürgen ; Buntkowsky, Gerd ; Zhuo, Fangping
Art des Eintrags: Bibliographie
Titel: Effect of temperature on dislocation-tuned dielectricity and piezoelectricity in single-crystal BaTiO3
Sprache: Englisch
Publikationsjahr: 11 März 2024
Verlag: AIP Publishing
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Applied Physics Letters
Jahrgang/Volume einer Zeitschrift: 124
DOI: 10.1063/5.0191394
Kurzbeschreibung (Abstract):

The pinning-controlled mobility of ferroelectric/ferroelastic domain walls is an important part of managing polarization switching and deter- mining the final properties of ferroelectric and piezoelectric materials. Here, we assess the impact of temperature on dislocation-induced domain wall pinning as well as on dislocation-tuned dielectric and piezoelectric response in barium titanate single crystals. Our solid-state nuclear magnetic resonance spectroscopy results indicate that the entire sample exclusively permits in-plane domains, with their distribution remaining insensitive to temperature changes below the Curie temperature (TC ). The domain wall pinning field monotonically decreases with increasing temperature up to TC , as evidenced by a combination of experimental observations and phase-field simulations. Our work high- lights the promising potential of dislocation engineering in controlling domain wall mobility within bulk ferroelectrics.

Zusätzliche Informationen:

Artikel-ID: 112904

Fachbereich(e)/-gebiet(e): 11 Fachbereich Material- und Geowissenschaften
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Fachgebiet Nichtmetallisch-Anorganische Werkstoffe
07 Fachbereich Chemie
07 Fachbereich Chemie > Eduard Zintl-Institut
07 Fachbereich Chemie > Eduard Zintl-Institut > Fachgebiet Physikalische Chemie
Hinterlegungsdatum: 12 Mär 2024 06:22
Letzte Änderung: 12 Mär 2024 06:36
PPN: 516226673
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