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All-optical spatio-temporal control of electron emission from SiO₂ nanospheres with femtosecond two-color laser fields

Liu, Qingcao ; Zherebtsov, Sergey ; Seiffert, Lennart ; Skruszewicz, Slawomir ; Zietlow, Dominik ; Ahn, Seongjin ; Rupp, Philipp ; Wnuk, Pawel ; Sun, Shaohua ; Kessel, Alexander ; Trushin, Sergei ; Schlander, Annika ; Kim, Dongeon ; Rühl, Eckart ; Ciappina, Marcelo F. ; Tiggesbäumker, Josef ; Gallei, Markus ; Fennel, Thomas ; Kling, Matthias F. (2019)
All-optical spatio-temporal control of electron emission from SiO₂ nanospheres with femtosecond two-color laser fields.
In: New Journal of Physics, 21 (7)
doi: 10.1088/1367-2630/ab26c1
Artikel, Bibliographie

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Kurzbeschreibung (Abstract)

Field localization by nanostructures illuminated with laser pulses of well-defined waveform enables spatio-temporal tailoring of the near-fields for sub-cycle control of electron dynamics at the nanoscale. Here, we apply intense linearly-polarized two-color laser pulses for all-optical control of the highest energy electron emission from SiO₂ nanoparticles. For the size regime where light propagation effects become important, we demonstrate the possibility to control the preferential emission angle of a considerable fraction of the fastest electrons by varying the relative phase of the two-color field. Trajectory based semi-classical simulations show that for the investigated nanoparticle size range the directional steering can be attributed to the two-color effect on the electron trajectories, while the accompanied modification of the spatial distribution of the ionization rate on the nanoparticle surface has only a minor effect.

Typ des Eintrags: Artikel
Erschienen: 2019
Autor(en): Liu, Qingcao ; Zherebtsov, Sergey ; Seiffert, Lennart ; Skruszewicz, Slawomir ; Zietlow, Dominik ; Ahn, Seongjin ; Rupp, Philipp ; Wnuk, Pawel ; Sun, Shaohua ; Kessel, Alexander ; Trushin, Sergei ; Schlander, Annika ; Kim, Dongeon ; Rühl, Eckart ; Ciappina, Marcelo F. ; Tiggesbäumker, Josef ; Gallei, Markus ; Fennel, Thomas ; Kling, Matthias F.
Art des Eintrags: Bibliographie
Titel: All-optical spatio-temporal control of electron emission from SiO₂ nanospheres with femtosecond two-color laser fields
Sprache: Englisch
Publikationsjahr: 1 Juli 2019
Ort: London
Verlag: IOP Publishing
Titel der Zeitschrift, Zeitung oder Schriftenreihe: New Journal of Physics
Jahrgang/Volume einer Zeitschrift: 21
(Heft-)Nummer: 7
Kollation: 9 Seiten
DOI: 10.1088/1367-2630/ab26c1
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Kurzbeschreibung (Abstract):

Field localization by nanostructures illuminated with laser pulses of well-defined waveform enables spatio-temporal tailoring of the near-fields for sub-cycle control of electron dynamics at the nanoscale. Here, we apply intense linearly-polarized two-color laser pulses for all-optical control of the highest energy electron emission from SiO₂ nanoparticles. For the size regime where light propagation effects become important, we demonstrate the possibility to control the preferential emission angle of a considerable fraction of the fastest electrons by varying the relative phase of the two-color field. Trajectory based semi-classical simulations show that for the investigated nanoparticle size range the directional steering can be attributed to the two-color effect on the electron trajectories, while the accompanied modification of the spatial distribution of the ionization rate on the nanoparticle surface has only a minor effect.

Freie Schlagworte: ultrafast nanophysics, two-color laser fields, spatio-temporal control, dielectric nanospheres
ID-Nummer: Artikel-ID: 073011
Sachgruppe der Dewey Dezimalklassifikatin (DDC): 500 Naturwissenschaften und Mathematik > 540 Chemie
Fachbereich(e)/-gebiet(e): 07 Fachbereich Chemie
07 Fachbereich Chemie > Ernst-Berl-Institut
07 Fachbereich Chemie > Ernst-Berl-Institut > Fachgebiet Makromolekulare Chemie
Hinterlegungsdatum: 14 Feb 2024 08:59
Letzte Änderung: 14 Feb 2024 08:59
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