Umo, N. S. ; Ullrich, R. ; Maters, E. C. ; Steinke, I. ; Benker, N. ; Höhler, K. ; Wagner, R. ; Weidler, P. G. ; Hoshyaripour, G. A. ; Kiselev, A. ; Kueppers, U. ; Kandler, K. ; Dingwell, D. B. ; Leisner, T. ; Möhler, O. (2024)
The Influence of Chemical and Mineral Compositions on the Parameterization of Immersion Freezing by Volcanic Ash Particles.
In: Journal of Geophysical Research: Atmospheres, 2021, 126 (17)
doi: 10.26083/tuprints-00020979
Artikel, Zweitveröffentlichung, Verlagsversion
 | Es ist eine neuere Version dieses Eintrags verfügbar. |
Kurzbeschreibung (Abstract)
Volcanic ash (VA) from explosive eruptions contributes to aerosol loadings in the atmosphere. Aside from the negative impact of VA on air quality and aviation, these particles can alter the optical and microphysical properties of clouds by triggering ice formation, thereby influencing precipitation and climate. Depending on the volcano and eruption style, VA displays a wide range of different physical, chemical, and mineralogical properties. Here, we present a unique data set on the ice nucleation activity of 15 VA samples obtained from different volcanoes worldwide. The ice nucleation activities of these samples were studied in the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) cloud simulation chamber as well as with the Ice Nucleation Spectrometer of the Karlsruhe Institute of Technology (INSEKT). All VA particles nucleated ice in the immersion freezing mode from 263 to 238K with ice nucleation active site (INAS) densities ranging from ∼10⁵ to 10¹¹ m⁻², respectively. The variabilities observed among the VA samples, at any given temperature, range over 3.5 orders of magnitude. The ice‐nucleating abilities of VA samples correlate to varying degrees with their bulk pyroxene and plagioclase contents as a function of temperature. We combined our new data set with existing literature data to develop an improved ice nucleation parameterization for natural VA in the immersion freezing mode. This should be useful for modeling the impact of VA on clouds.
| Typ des Eintrags: | Artikel |
|---|---|
| Erschienen: | 2024 |
| Autor(en): | Umo, N. S. ; Ullrich, R. ; Maters, E. C. ; Steinke, I. ; Benker, N. ; Höhler, K. ; Wagner, R. ; Weidler, P. G. ; Hoshyaripour, G. A. ; Kiselev, A. ; Kueppers, U. ; Kandler, K. ; Dingwell, D. B. ; Leisner, T. ; Möhler, O. |
| Art des Eintrags: | Zweitveröffentlichung |
| Titel: | The Influence of Chemical and Mineral Compositions on the Parameterization of Immersion Freezing by Volcanic Ash Particles |
| Sprache: | Englisch |
| Publikationsjahr: | 13 Februar 2024 |
| Ort: | Darmstadt |
| Publikationsdatum der Erstveröffentlichung: | 2021 |
| Ort der Erstveröffentlichung: | Hoboken |
| Verlag: | Wiley |
| Titel der Zeitschrift, Zeitung oder Schriftenreihe: | Journal of Geophysical Research: Atmospheres |
| Jahrgang/Volume einer Zeitschrift: | 126 |
| (Heft-)Nummer: | 17 |
| Kollation: | 27 Seiten |
| DOI: | 10.26083/tuprints-00020979 |
| URL / URN: | https://tuprints.ulb.tu-darmstadt.de/20979 |
| Zugehörige Links: | |
| Herkunft: | Zweitveröffentlichung DeepGreen |
| Kurzbeschreibung (Abstract): | Volcanic ash (VA) from explosive eruptions contributes to aerosol loadings in the atmosphere. Aside from the negative impact of VA on air quality and aviation, these particles can alter the optical and microphysical properties of clouds by triggering ice formation, thereby influencing precipitation and climate. Depending on the volcano and eruption style, VA displays a wide range of different physical, chemical, and mineralogical properties. Here, we present a unique data set on the ice nucleation activity of 15 VA samples obtained from different volcanoes worldwide. The ice nucleation activities of these samples were studied in the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) cloud simulation chamber as well as with the Ice Nucleation Spectrometer of the Karlsruhe Institute of Technology (INSEKT). All VA particles nucleated ice in the immersion freezing mode from 263 to 238K with ice nucleation active site (INAS) densities ranging from ∼10⁵ to 10¹¹ m⁻², respectively. The variabilities observed among the VA samples, at any given temperature, range over 3.5 orders of magnitude. The ice‐nucleating abilities of VA samples correlate to varying degrees with their bulk pyroxene and plagioclase contents as a function of temperature. We combined our new data set with existing literature data to develop an improved ice nucleation parameterization for natural VA in the immersion freezing mode. This should be useful for modeling the impact of VA on clouds. |
| Freie Schlagworte: | aerosol, chemical composition, cloud chamber, ice nucleation, mineralogy, mixed‐phase clouds, parameterization, volcanic ash |
| ID-Nummer: | Artikel-ID: e2020JD033356 |
| Status: | Verlagsversion |
| URN: | urn:nbn:de:tuda-tuprints-209791 |
| Sachgruppe der Dewey Dezimalklassifikatin (DDC): | 500 Naturwissenschaften und Mathematik > 550 Geowissenschaften |
| Fachbereich(e)/-gebiet(e): | 11 Fachbereich Material- und Geowissenschaften 11 Fachbereich Material- und Geowissenschaften > Geowissenschaften 11 Fachbereich Material- und Geowissenschaften > Geowissenschaften > Fachgebiet Atmosphärisches Aerosol |
| Hinterlegungsdatum: | 13 Feb 2024 13:32 |
| Letzte Änderung: | 14 Feb 2024 08:00 |
| PPN: | |
| Zugehörige Links: | |
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| Suche nach Titel in: | TUfind oder in Google |
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- The Influence of Chemical and Mineral Compositions on the Parameterization of Immersion Freezing by Volcanic Ash Particles. (deposited 13 Feb 2024 13:32) [Gegenwärtig angezeigt]
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