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Low-frequency spin dynamics as probed by ⁶³Cu and ¹⁹⁹Hg NMR in HgBa₂CuO₄₊δ superconductors with different oxygen content

Gippius, Andrei Andreevich ; Antipov, Evgeny V. ; Hoffmann, W. ; Lüders, Klaus ; Buntkowsky, Gerd (2023)
Low-frequency spin dynamics as probed by ⁶³Cu and ¹⁹⁹Hg NMR in HgBa₂CuO₄₊δ superconductors with different oxygen content.
In: Physical Review B, 1999, 59 (1)
doi: 10.26083/tuprints-00024240
Artikel, Zweitveröffentlichung, Verlagsversion

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Kurzbeschreibung (Abstract)

⁶³Cu and ¹⁹⁹Hg nuclear magnetic resonance was performed on a series of powder HgBa₂CuO₄₊δ samples with different oxygen content δ in order to study the influence of oxygen doping on the spin dynamics in the normal and superconducting state. The spin-lattice relaxation time T₁ of ¹⁹⁹Hg and ⁶³Cu nuclei were measured over a wide range of temperature at different orientations of the crystallites with respect to the magnetic field. For the optimally doped sample (Tc=96 K) we compared our experimental results to numerical calculations of the spin-lattice relaxation rate as a function of temperature below Tc for several types of the order parameter symmetry: isotropic s wave, anisotropic s wave without nodes, s wave with nodes, and d wave, using the different values of the gap parameter 2Δ/kBTc within the AF fluctuation model. The comparison with our experimental relaxation data shows that for ¹⁹⁹Hg nuclei in the orientation B₀∥(a,b) plane as well as for ⁶³Cu nuclei in both orientations, B₀∥(a,b) plane and B₀∥c axis, the experimental results are in coincidence with the dx2₋y2-wave symmetry with the gap parameter 2Δ/kBTc=7.02.

Typ des Eintrags: Artikel
Erschienen: 2023
Autor(en): Gippius, Andrei Andreevich ; Antipov, Evgeny V. ; Hoffmann, W. ; Lüders, Klaus ; Buntkowsky, Gerd
Art des Eintrags: Zweitveröffentlichung
Titel: Low-frequency spin dynamics as probed by ⁶³Cu and ¹⁹⁹Hg NMR in HgBa₂CuO₄₊δ superconductors with different oxygen content
Sprache: Englisch
Publikationsjahr: 2023
Ort: Darmstadt
Publikationsdatum der Erstveröffentlichung: 1999
Verlag: American Physical Society
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Physical Review B
Jahrgang/Volume einer Zeitschrift: 59
(Heft-)Nummer: 1
DOI: 10.26083/tuprints-00024240
URL / URN: https://tuprints.ulb.tu-darmstadt.de/24240
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Herkunft: Zweitveröffentlichungsservice
Kurzbeschreibung (Abstract):

⁶³Cu and ¹⁹⁹Hg nuclear magnetic resonance was performed on a series of powder HgBa₂CuO₄₊δ samples with different oxygen content δ in order to study the influence of oxygen doping on the spin dynamics in the normal and superconducting state. The spin-lattice relaxation time T₁ of ¹⁹⁹Hg and ⁶³Cu nuclei were measured over a wide range of temperature at different orientations of the crystallites with respect to the magnetic field. For the optimally doped sample (Tc=96 K) we compared our experimental results to numerical calculations of the spin-lattice relaxation rate as a function of temperature below Tc for several types of the order parameter symmetry: isotropic s wave, anisotropic s wave without nodes, s wave with nodes, and d wave, using the different values of the gap parameter 2Δ/kBTc within the AF fluctuation model. The comparison with our experimental relaxation data shows that for ¹⁹⁹Hg nuclei in the orientation B₀∥(a,b) plane as well as for ⁶³Cu nuclei in both orientations, B₀∥(a,b) plane and B₀∥c axis, the experimental results are in coincidence with the dx2₋y2-wave symmetry with the gap parameter 2Δ/kBTc=7.02.

Status: Verlagsversion
URN: urn:nbn:de:tuda-tuprints-242406
Sachgruppe der Dewey Dezimalklassifikatin (DDC): 500 Naturwissenschaften und Mathematik > 530 Physik
500 Naturwissenschaften und Mathematik > 540 Chemie
Fachbereich(e)/-gebiet(e): 07 Fachbereich Chemie
07 Fachbereich Chemie > Eduard Zintl-Institut
07 Fachbereich Chemie > Eduard Zintl-Institut > Fachgebiet Physikalische Chemie
Hinterlegungsdatum: 12 Jul 2023 12:48
Letzte Änderung: 01 Aug 2024 09:05
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