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Catchment Soil Properties Affect Metal(loid) Enrichment in Reservoir Sediments of German Low Mountain Regions

Hahn, Jens ; Bui, Thanh ; Kessler, Mathias ; Weber, Collin J. ; Beier, Thomas ; Mildenberger, Antje ; Traub, Martina ; Opp, Christian (2022)
Catchment Soil Properties Affect Metal(loid) Enrichment in Reservoir Sediments of German Low Mountain Regions.
In: Applied Sciences, 2022, 12 (5)
doi: 10.26083/tuprints-00022526
Artikel, Zweitveröffentlichung, Verlagsversion

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Kurzbeschreibung (Abstract)

Sediment management is a fundamental part of reservoir operation, but it is often complicated by metal(loid) enrichment in sediments. Knowledge concerning the sources of potential contaminants is therefore of important significance. To address this issue, the concentrations and the mobile fractions of metal(loid)s were determined in the sediments and the respective catchment areas of six reservoirs. The results indicate that reservoirs generally have a high potential for contaminated sediment accumulation due to preferential deposition of fine particles. The median values of the element-specific enrichment factor (EF) demonstrates slight enrichments of arsenic (EF: 3.4), chromium (EF: 2.8), and vanadium (EF: 2.9) for reservoir sediments. The enrichments of cadmium (EF: 8.2), manganese (EF: 3.9), nickel (EF: 4.8), and zinc (EF: 5.0) are significantly higher. This is enabled by a diffuse element release from the soils into the impounded streams, which is particularly favored by soil acidity. Leaching from the catchment soils partially enriches elements in stream sediments before their fine-grained portions in particular are deposited as reservoir sediment. We assume that this effect is of high relevance especially for reservoirs impounding small streams with forested catchments and weakly acid buffering parent material of soil formation.

Typ des Eintrags: Artikel
Erschienen: 2022
Autor(en): Hahn, Jens ; Bui, Thanh ; Kessler, Mathias ; Weber, Collin J. ; Beier, Thomas ; Mildenberger, Antje ; Traub, Martina ; Opp, Christian
Art des Eintrags: Zweitveröffentlichung
Titel: Catchment Soil Properties Affect Metal(loid) Enrichment in Reservoir Sediments of German Low Mountain Regions
Sprache: Englisch
Publikationsjahr: 2022
Ort: Darmstadt
Publikationsdatum der Erstveröffentlichung: 2022
Verlag: MDPI
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Applied Sciences
Jahrgang/Volume einer Zeitschrift: 12
(Heft-)Nummer: 5
Kollation: 15 Seiten
DOI: 10.26083/tuprints-00022526
URL / URN: https://tuprints.ulb.tu-darmstadt.de/22526
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Herkunft: Zweitveröffentlichungsservice
Kurzbeschreibung (Abstract):

Sediment management is a fundamental part of reservoir operation, but it is often complicated by metal(loid) enrichment in sediments. Knowledge concerning the sources of potential contaminants is therefore of important significance. To address this issue, the concentrations and the mobile fractions of metal(loid)s were determined in the sediments and the respective catchment areas of six reservoirs. The results indicate that reservoirs generally have a high potential for contaminated sediment accumulation due to preferential deposition of fine particles. The median values of the element-specific enrichment factor (EF) demonstrates slight enrichments of arsenic (EF: 3.4), chromium (EF: 2.8), and vanadium (EF: 2.9) for reservoir sediments. The enrichments of cadmium (EF: 8.2), manganese (EF: 3.9), nickel (EF: 4.8), and zinc (EF: 5.0) are significantly higher. This is enabled by a diffuse element release from the soils into the impounded streams, which is particularly favored by soil acidity. Leaching from the catchment soils partially enriches elements in stream sediments before their fine-grained portions in particular are deposited as reservoir sediment. We assume that this effect is of high relevance especially for reservoirs impounding small streams with forested catchments and weakly acid buffering parent material of soil formation.

Freie Schlagworte: reservoir, soil, catchment, sediment, metals, trace elements, enrichment, element mobility
Status: Verlagsversion
URN: urn:nbn:de:tuda-tuprints-225260
Sachgruppe der Dewey Dezimalklassifikatin (DDC): 500 Naturwissenschaften und Mathematik > 550 Geowissenschaften
Fachbereich(e)/-gebiet(e): 11 Fachbereich Material- und Geowissenschaften
11 Fachbereich Material- und Geowissenschaften > Geowissenschaften
11 Fachbereich Material- und Geowissenschaften > Geowissenschaften > Fachgebiet Bodenmineralogie und Bodenchemie
Hinterlegungsdatum: 10 Nov 2022 13:09
Letzte Änderung: 11 Nov 2022 08:29
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