Nowroozi, Mohammad Ali ; Waidha, Aamir Iqbal ; Jacob, Martine ; Aken, Peter A. van ; Predel, Felicitas ; Ensinger, Wolfgang ; Clemens, Oliver (2022)
Towards Recycling of LLZO Solid Electrolyte Exemplarily Performed on LFP/LLZO/LTO Cells.
In: ChemistryOpen, 2022, 11 (3)
doi: 10.26083/tuprints-00021454
Artikel, Zweitveröffentlichung, Verlagsversion

Kurzbeschreibung (Abstract)

All-solid-state lithium ion batteries (ASS-LIBs) are promising due to their safety and higher energy density as compared to that of conventional LIBs. Over the next few decades, tremendous amounts of spent ASS-LIBs will reach the end of their cycle life and would require recycling in order to address the waste management issue along with reduced exploitation of rare elements. So far, only very limited studies have been conducted on recycling of ASS-LIBS. Herein, we investigate the recycling of the Li₇La₃Zr₂O₁₂ (LLZO) solid-state electrolyte in a LiFePO₄/LLZO/ Li₄Ti₅O₁₂ system using a hydrometallurgical approach. Our results show that different concentration of the leaching solutions can significantly influence the final product of the recycling process. However, it was possible to recover relatively pure La₂O₃ and ZrO₂ to re-synthesize the cubic LLZO phase, whose high purity was confirmed by XRD measurements.

Typ des Eintrags:	Artikel
Erschienen:	2022
Autor(en):	Nowroozi, Mohammad Ali ; Waidha, Aamir Iqbal ; Jacob, Martine ; Aken, Peter A. van ; Predel, Felicitas ; Ensinger, Wolfgang ; Clemens, Oliver
Art des Eintrags:	Zweitveröffentlichung
Titel:	Towards Recycling of LLZO Solid Electrolyte Exemplarily Performed on LFP/LLZO/LTO Cells
Sprache:	Englisch
Publikationsjahr:	2022
Publikationsdatum der Erstveröffentlichung:	2022
Verlag:	Wiley
Titel der Zeitschrift, Zeitung oder Schriftenreihe:	ChemistryOpen
Jahrgang/Volume einer Zeitschrift:	11
(Heft-)Nummer:	3
Kollation:	13 Seiten
DOI:	10.26083/tuprints-00021454
URL / URN:	https://tuprints.ulb.tu-darmstadt.de/21454
Zugehörige Links:	Verlags-DOI Verlag Identisches Werk
Herkunft:	Zweitveröffentlichung aus gefördertem Golden Open Access
Kurzbeschreibung (Abstract):	All-solid-state lithium ion batteries (ASS-LIBs) are promising due to their safety and higher energy density as compared to that of conventional LIBs. Over the next few decades, tremendous amounts of spent ASS-LIBs will reach the end of their cycle life and would require recycling in order to address the waste management issue along with reduced exploitation of rare elements. So far, only very limited studies have been conducted on recycling of ASS-LIBS. Herein, we investigate the recycling of the Li₇La₃Zr₂O₁₂ (LLZO) solid-state electrolyte in a LiFePO₄/LLZO/ Li₄Ti₅O₁₂ system using a hydrometallurgical approach. Our results show that different concentration of the leaching solutions can significantly influence the final product of the recycling process. However, it was possible to recover relatively pure La₂O₃ and ZrO₂ to re-synthesize the cubic LLZO phase, whose high purity was confirmed by XRD measurements.
Alternatives oder übersetztes Abstract:	Alternatives Abstract Sprache Recycling of solid-state batteries, which are expected to become extremely important in the energy industry over the next decade, is often very complex due to the solid electrolyte. Here, recycling of all-solid-state lithium ion batteries has been approached by a combination of mechanical/hydrometallurgical methods. Promising results confirm the recovering of the solid-electrolyte. Englisch
Status:	Verlagsversion
URN:	urn:nbn:de:tuda-tuprints-214544
Sachgruppe der Dewey Dezimalklassifikatin (DDC):	500 Naturwissenschaften und Mathematik > 540 Chemie 600 Technik, Medizin, angewandte Wissenschaften > 620 Ingenieurwissenschaften und Maschinenbau
Fachbereich(e)/-gebiet(e):	11 Fachbereich Material- und Geowissenschaften 11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft 11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Fachgebiet Materialanalytik
Hinterlegungsdatum:	10 Jun 2022 11:12
Letzte Änderung:	13 Jun 2022 06:10
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Verfügbare Versionen dieses Eintrags

• Towards Recycling of LLZO Solid Electrolyte Exemplarily Performed on LFP/LLZO/LTO Cells. (deposited 10 Jun 2022 11:12) [Gegenwärtig angezeigt]
  • Towards Recycling of LLZO Solid Electrolyte Exemplarily Performed on LFP/LLZO/LTO Cells. (deposited 02 Aug 2024 12:41)

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