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Large electrocaloric effect with ultrawide temperature span in Na1/2Bi1/2TiO3-based lead-free ceramics

Wei, Qiumei ; Fulanovic, Lovro ; Kodumudi Venkataraman, Lalitha ; Zheng, Mupeng ; Hou, Yudong ; Zhu, Mankang ; Liu, Linjing ; Chang, Yunfei ; Xue, Rui (2022)
Large electrocaloric effect with ultrawide temperature span in Na1/2Bi1/2TiO3-based lead-free ceramics.
In: Journal of the American Ceramic Society, 105 (5)
doi: 10.1111/jace.18291
Artikel, Bibliographie

Kurzbeschreibung (Abstract)

Innovative cooling technologies are recognized by many industries as a crucial part of their system design. A large electrocaloric effect (ECE) and extended working temperature are the key issues hindering the realization of electrocaloric refrigeration technology. In this work, large ECE (ΔT = 0.8–0.9◦C @ 4 kV/mm) with an ultrawide temperature span from 30 to 120◦C is noted for lead-free (Na1/2Bi1/2)0.80Sr0.20(Zn1/3Nb2/3)xTi1-xO3 ceramics. The excellent ECE performance can be ascribed to the evolution of polar nanoregions. Our work suggests that this material is promising for applications in solid-state refrigeration systems with a broad range of operating temperatures.

Typ des Eintrags: Artikel
Erschienen: 2022
Autor(en): Wei, Qiumei ; Fulanovic, Lovro ; Kodumudi Venkataraman, Lalitha ; Zheng, Mupeng ; Hou, Yudong ; Zhu, Mankang ; Liu, Linjing ; Chang, Yunfei ; Xue, Rui
Art des Eintrags: Bibliographie
Titel: Large electrocaloric effect with ultrawide temperature span in Na1/2Bi1/2TiO3-based lead-free ceramics
Sprache: Englisch
Publikationsjahr: 2 Mai 2022
Verlag: Wiley
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Journal of the American Ceramic Society
Jahrgang/Volume einer Zeitschrift: 105
(Heft-)Nummer: 5
DOI: 10.1111/jace.18291
Kurzbeschreibung (Abstract):

Innovative cooling technologies are recognized by many industries as a crucial part of their system design. A large electrocaloric effect (ECE) and extended working temperature are the key issues hindering the realization of electrocaloric refrigeration technology. In this work, large ECE (ΔT = 0.8–0.9◦C @ 4 kV/mm) with an ultrawide temperature span from 30 to 120◦C is noted for lead-free (Na1/2Bi1/2)0.80Sr0.20(Zn1/3Nb2/3)xTi1-xO3 ceramics. The excellent ECE performance can be ascribed to the evolution of polar nanoregions. Our work suggests that this material is promising for applications in solid-state refrigeration systems with a broad range of operating temperatures.

Freie Schlagworte: Dielectric, electrocaloric effect, lead–free ferroelectrics, Na0.5Bi0.5TiO3, relaxor behavior
Fachbereich(e)/-gebiet(e): 11 Fachbereich Material- und Geowissenschaften
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Fachgebiet Nichtmetallisch-Anorganische Werkstoffe
Hinterlegungsdatum: 11 Mär 2022 11:56
Letzte Änderung: 11 Mär 2022 11:56
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