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Design of a 1 MWth Pilot Plant for Chemical Looping Gasification of Biogenic Residues

Marx, Falko ; Dieringer, Paul ; Ströhle, Jochen ; Epple, Bernd (2022)
Design of a 1 MWth Pilot Plant for Chemical Looping Gasification of Biogenic Residues.
In: Energies, 2021, 14 (9)
doi: 10.26083/tuprints-00019522
Artikel, Zweitveröffentlichung, Verlagsversion

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Kurzbeschreibung (Abstract)

Chemical looping gasification (CLG) is a promising process for the thermochemical solid to liquid conversion route using lattice oxygen, provided by a solid oxygen carrier material, to produce a nitrogen free synthesis gas. Recent advances in lab-scale experiments show that CLG with biomass has the possibility to produce a carbon neutral synthesis gas. However, all experiments have been conducted in externally heated units, not enabling autothermal operation. In this study, the modification of an existing pilot plant for demonstrating autothermal operation of CLG is described. Energy and mass balances are calculated using a validated chemical looping combustion process model extended for biomass gasification. Based on six operational cases, adaptations of the pilot plant are designed and changes discussed. A reactor configuration using two circulating fluidized bed reactors with internal solid circulation in the air reactor is proposed and a suitable operating strategy devised. The resulting experimental unit enables a reasonable range of operational parameters within restrictions imposed from autothermal operation.

Typ des Eintrags: Artikel
Erschienen: 2022
Autor(en): Marx, Falko ; Dieringer, Paul ; Ströhle, Jochen ; Epple, Bernd
Art des Eintrags: Zweitveröffentlichung
Titel: Design of a 1 MWth Pilot Plant for Chemical Looping Gasification of Biogenic Residues
Sprache: Englisch
Publikationsjahr: 2022
Ort: Darmstadt
Publikationsdatum der Erstveröffentlichung: 2021
Verlag: MDPI
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Energies
Jahrgang/Volume einer Zeitschrift: 14
(Heft-)Nummer: 9
Kollation: 25 Seiten
DOI: 10.26083/tuprints-00019522
URL / URN: https://tuprints.ulb.tu-darmstadt.de/19522
Zugehörige Links:
Herkunft: Zweitveröffentlichung DeepGreen
Kurzbeschreibung (Abstract):

Chemical looping gasification (CLG) is a promising process for the thermochemical solid to liquid conversion route using lattice oxygen, provided by a solid oxygen carrier material, to produce a nitrogen free synthesis gas. Recent advances in lab-scale experiments show that CLG with biomass has the possibility to produce a carbon neutral synthesis gas. However, all experiments have been conducted in externally heated units, not enabling autothermal operation. In this study, the modification of an existing pilot plant for demonstrating autothermal operation of CLG is described. Energy and mass balances are calculated using a validated chemical looping combustion process model extended for biomass gasification. Based on six operational cases, adaptations of the pilot plant are designed and changes discussed. A reactor configuration using two circulating fluidized bed reactors with internal solid circulation in the air reactor is proposed and a suitable operating strategy devised. The resulting experimental unit enables a reasonable range of operational parameters within restrictions imposed from autothermal operation.

Freie Schlagworte: chemical looping, biomass, gasification, fluidized bed, autothermal, pilot plant
Status: Verlagsversion
URN: urn:nbn:de:tuda-tuprints-195223
Sachgruppe der Dewey Dezimalklassifikatin (DDC): 600 Technik, Medizin, angewandte Wissenschaften > 600 Technik
Fachbereich(e)/-gebiet(e): 16 Fachbereich Maschinenbau
16 Fachbereich Maschinenbau > Institut für Energiesysteme und Energietechnik (EST)
Hinterlegungsdatum: 31 Jan 2022 13:05
Letzte Änderung: 06 Dez 2023 09:26
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