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Simulation of the Carbonate Looping Process for Post-Combustion CO2 Capture from a Coal-Fired Power Plant

Ströhle, Jochen ; Lasheras, Ana ; Galloy, Alexander ; Epple, Bernd (2009)
Simulation of the Carbonate Looping Process for Post-Combustion CO2 Capture from a Coal-Fired Power Plant.
In: Chemical Engineering & Technology, 32 (3)
doi: 10.1002/ceat.200800569
Article, Bibliographie

Abstract

The present contribution focuses on the carbonate looping process, i.e., post-combustion CO2 capture by means of CaO containing solid sorbents in a system of two circulating fluidized bed reactors. Material and energy balances were performed using the ASPEN PLUSTM software. Two different modeling approaches are applied to the carbonator. First, the entire active fraction of CaO is assumed to be converted; second, the CO2 absorption efficiency in the circulating fluidized bed is calculated using an analytical 1D model for fast fluidization. The absorption of SO2 by CaO is taken into account. The overall plant efficiency depends on the mass flows of fresh limestone and circulating CaO. The process is shown to be economically feasible, having low energy penalties in comparison with other CO2 capture technologies and it seems to be suited for retro-fitting existing power plants.

Item Type: Article
Erschienen: 2009
Creators: Ströhle, Jochen ; Lasheras, Ana ; Galloy, Alexander ; Epple, Bernd
Type of entry: Bibliographie
Title: Simulation of the Carbonate Looping Process for Post-Combustion CO2 Capture from a Coal-Fired Power Plant
Language: English
Date: March 2009
Journal or Publication Title: Chemical Engineering & Technology
Volume of the journal: 32
Issue Number: 3
DOI: 10.1002/ceat.200800569
URL / URN: https://doi.org/10.1002/ceat.200800569
Abstract:

The present contribution focuses on the carbonate looping process, i.e., post-combustion CO2 capture by means of CaO containing solid sorbents in a system of two circulating fluidized bed reactors. Material and energy balances were performed using the ASPEN PLUSTM software. Two different modeling approaches are applied to the carbonator. First, the entire active fraction of CaO is assumed to be converted; second, the CO2 absorption efficiency in the circulating fluidized bed is calculated using an analytical 1D model for fast fluidization. The absorption of SO2 by CaO is taken into account. The overall plant efficiency depends on the mass flows of fresh limestone and circulating CaO. The process is shown to be economically feasible, having low energy penalties in comparison with other CO2 capture technologies and it seems to be suited for retro-fitting existing power plants.

Uncontrolled Keywords: Carbonate looping, Circulating fluidized beds, CO2 capture, Simulation
Divisions: 16 Department of Mechanical Engineering
16 Department of Mechanical Engineering > Institut für Energiesysteme und Energietechnik (EST)
Date Deposited: 08 Feb 2018 07:17
Last Modified: 08 Feb 2018 07:17
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