Waidha, Aamir Iqbal ; Salihovic, Amila ; Jacob, Martine ; Vanita, Vanita ; Aktekin, Burak ; Brix, Kristina ; Wissel, Kerstin ; Kautenburger, Ralf ; Janek, Jürgen ; Ensinger, Wolfgang ; Clemens, Oliver (2023)
Recycling of All‐Solid‐State Li‐ion Batteries: A Case Study of the Separation of Individual Components Within a System Composed of LTO, LLZTO and NMC.
In: ChemSusChem, 16 (13)
doi: 10.1002/cssc.202202361
Article, Bibliographie
This is the latest version of this item.
Abstract
With the current global projection of over 130 million electric vehicles (EVs), there soon will be a need for battery waste management. Especially for all‐solid‐state lithium‐ion batteries (lithium ASSBs), aspects of waste management and circular economy have not been addressed so far. Within such ASSBs, the use of solid‐electrolytes like garnet‐type Li₆.₅La₃Zr₁.₅Ta₀.₅O₁₂ (LLZTO) may shift focus on strategies to recover not only the transition metal elements but also elements like La/Zr/Ta. In this work, we present a two‐step recycling approach using citric acid as the leaching agent to separate and recover the individual components of a model cell comprising of Li₄Ti₅O₁₂ (LTO) anode, Li₆.₅La₃Zr₁.₅Ta₀.₅O₁₂ (LLZTO) garnet electrolyte and LiNi₁/₃Mn₁/₃Co₁/₃O₂ (NMC) cathode. We observe that by adjusting the concentration of citric acid, it was possible to separate the materials from each other without strong mixing of individual phases and also to maintain their principle performance characteristics. Thus, the process developed has a potential for upscaling and can guide towards considering separation capability of battery components in the development of lithium ASSBs.
| Item Type: | Article |
|---|---|
| Erschienen: | 2023 |
| Creators: | Waidha, Aamir Iqbal ; Salihovic, Amila ; Jacob, Martine ; Vanita, Vanita ; Aktekin, Burak ; Brix, Kristina ; Wissel, Kerstin ; Kautenburger, Ralf ; Janek, Jürgen ; Ensinger, Wolfgang ; Clemens, Oliver |
| Type of entry: | Bibliographie |
| Title: | Recycling of All‐Solid‐State Li‐ion Batteries: A Case Study of the Separation of Individual Components Within a System Composed of LTO, LLZTO and NMC |
| Language: | English |
| Date: | 2023 |
| Place of Publication: | Darmstadt |
| Publisher: | Wiley-VCH |
| Journal or Publication Title: | ChemSusChem |
| Volume of the journal: | 16 |
| Issue Number: | 13 |
| Collation: | 13 Seiten |
| DOI: | 10.1002/cssc.202202361 |
| Corresponding Links: | |
| Abstract: | With the current global projection of over 130 million electric vehicles (EVs), there soon will be a need for battery waste management. Especially for all‐solid‐state lithium‐ion batteries (lithium ASSBs), aspects of waste management and circular economy have not been addressed so far. Within such ASSBs, the use of solid‐electrolytes like garnet‐type Li₆.₅La₃Zr₁.₅Ta₀.₅O₁₂ (LLZTO) may shift focus on strategies to recover not only the transition metal elements but also elements like La/Zr/Ta. In this work, we present a two‐step recycling approach using citric acid as the leaching agent to separate and recover the individual components of a model cell comprising of Li₄Ti₅O₁₂ (LTO) anode, Li₆.₅La₃Zr₁.₅Ta₀.₅O₁₂ (LLZTO) garnet electrolyte and LiNi₁/₃Mn₁/₃Co₁/₃O₂ (NMC) cathode. We observe that by adjusting the concentration of citric acid, it was possible to separate the materials from each other without strong mixing of individual phases and also to maintain their principle performance characteristics. Thus, the process developed has a potential for upscaling and can guide towards considering separation capability of battery components in the development of lithium ASSBs. |
| Uncontrolled Keywords: | lithium-ion batteries, solid-state batteries, recycling, garnet, circular economy |
| Identification Number: | e202202361 |
| Additional Information: | This article also appears in: Solid State Batteries |
| Classification DDC: | 600 Technology, medicine, applied sciences > 660 Chemical engineering |
| Divisions: | 11 Department of Materials and Earth Sciences 11 Department of Materials and Earth Sciences > Material Science 11 Department of Materials and Earth Sciences > Material Science > Material Analytics |
| Date Deposited: | 02 Aug 2024 12:54 |
| Last Modified: | 02 Aug 2024 12:54 |
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| Suche nach Titel in: | TUfind oder in Google |
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Recycling of All‐Solid‐State Li‐ion Batteries: A Case Study of the Separation of Individual Components Within a System Composed of LTO, LLZTO and NMC. (deposited 07 Aug 2023 08:27)
- Recycling of All‐Solid‐State Li‐ion Batteries: A Case Study of the Separation of Individual Components Within a System Composed of LTO, LLZTO and NMC. (deposited 02 Aug 2024 12:54) [Currently Displayed]
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