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Towards Double Resonant Cavity Enhanced Second Harmonic Generation in Monolayer MoS₂

Shradha, Sai ; Abtahi, Fatemeh ; Gan, Ziyang ; Knopf, Heiko ; Fedotova, Anna ; Löchner, Franz J. F. ; George, Antony ; Pertsch, Thomas ; Turchanin, Andrey ; Eilenberger, Falk (2024)
Towards Double Resonant Cavity Enhanced Second Harmonic Generation in Monolayer MoS₂.
In: Advanced Optical Materials, 12 (6)
doi: 10.1002/adom.202300907
Article, Bibliographie

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Abstract

A characteristic property of monolayered transition metal dichalcogenides is their strong nonlinear response. While they display a high conversion efficiency per atomic layer, due to their low thickness, the absolute value of their nonlinear response remains low. Here enhancement of the second harmonic generation (SHG) of monolayer MoS₂ through the design, fabrication, and characterization of a monolithic microcavity, which aims to be double resonant at a fundamental wavelength of λ = 800 nm as well as its second harmonic, is demonstrated. The MoS₂ monolayers are embedded in such a cavity, with the aim to simultaneously enhance the light‐matter interaction at the excitation wavelength and the SHG from the monolayers. A resonance enhancement for the SHG process is achieved through the cavity.

Item Type: Article
Erschienen: 2024
Creators: Shradha, Sai ; Abtahi, Fatemeh ; Gan, Ziyang ; Knopf, Heiko ; Fedotova, Anna ; Löchner, Franz J. F. ; George, Antony ; Pertsch, Thomas ; Turchanin, Andrey ; Eilenberger, Falk
Type of entry: Bibliographie
Title: Towards Double Resonant Cavity Enhanced Second Harmonic Generation in Monolayer MoS₂
Language: English
Date: 23 February 2024
Place of Publication: Weinheim
Publisher: Wiley-VCH
Journal or Publication Title: Advanced Optical Materials
Volume of the journal: 12
Issue Number: 6
Collation: 6 Seiten
DOI: 10.1002/adom.202300907
Corresponding Links:
Abstract:

A characteristic property of monolayered transition metal dichalcogenides is their strong nonlinear response. While they display a high conversion efficiency per atomic layer, due to their low thickness, the absolute value of their nonlinear response remains low. Here enhancement of the second harmonic generation (SHG) of monolayer MoS₂ through the design, fabrication, and characterization of a monolithic microcavity, which aims to be double resonant at a fundamental wavelength of λ = 800 nm as well as its second harmonic, is demonstrated. The MoS₂ monolayers are embedded in such a cavity, with the aim to simultaneously enhance the light‐matter interaction at the excitation wavelength and the SHG from the monolayers. A resonance enhancement for the SHG process is achieved through the cavity.

Uncontrolled Keywords: microcavity, second harmonic generation, transition metal dichalcogenides
Identification Number: Artikel-ID: 2300907
Additional Information:

Special Section: Optical Metamaterials and Information Metamaterials

Classification DDC: 500 Science and mathematics > 530 Physics
500 Science and mathematics > 540 Chemistry
Divisions: 05 Department of Physics
05 Department of Physics > Institute for Condensed Matter Physics
05 Department of Physics > Institute for Condensed Matter Physics > Hybrid Quantum Systems
Date Deposited: 18 Jun 2024 06:48
Last Modified: 18 Jun 2024 06:48
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