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The influence of intra-droplet heat and mass transfer limitations in evaporation of binary hydrocarbon mixtures

Keller, P. ; Bader, A. ; Hasse, C. (2013)
The influence of intra-droplet heat and mass transfer limitations in evaporation of binary hydrocarbon mixtures.
In: International Journal of Heat and Mass Transfer, 67 (0)
doi: 10.1016/j.ijheatmasstransfer.2013.08.104
Artikel, Bibliographie

Kurzbeschreibung (Abstract)

The influence of intra-droplet heat and mass transfer limitations during the evaporation of binary hydro- carbon mixtures is investigated. Liquid transport processes are described with a 1D formulation (diffu- sion limit model – DLM) taking into account temporal and spatial gradients of the substance properties. The vapor liquid equilibrium is described with a c – u model and the activity coefficients are calculated using the NRTL approach. A suitably normalized segregation factor for each component based on the time-integrated evaporation rate is introduced and used for the analysis of n-heptane/n- decane and n-heptane/iso-octane droplets varying the ambient conditions and the initial liquid compo- sitions. Simulations with the DLM approach are compared to results obtained with a 0D model (rapid mixing model – RMM), which assumes homogeneous droplets in the infinite-diffusivity limit. Simulation results are also compared to experimental data where available. Biot numbers for heat and mass transfer as well as Lewis numbers for the liquid phase are evaluated and their differences are analyzed. A constant Lewis number based approach to calculate the liquid diffusion coefficients is investigated in detail as an alternative to the computationally expensive calculation of the individual diffusion coefficients at each inner droplet location. A suitable strategy to precompute the Lewis number as a function of temperature and composition is presented and the results are compared to the detailed calculations.

Typ des Eintrags: Artikel
Erschienen: 2013
Autor(en): Keller, P. ; Bader, A. ; Hasse, C.
Art des Eintrags: Bibliographie
Titel: The influence of intra-droplet heat and mass transfer limitations in evaporation of binary hydrocarbon mixtures
Sprache: Englisch
Publikationsjahr: 2013
Titel der Zeitschrift, Zeitung oder Schriftenreihe: International Journal of Heat and Mass Transfer
Jahrgang/Volume einer Zeitschrift: 67
(Heft-)Nummer: 0
DOI: 10.1016/j.ijheatmasstransfer.2013.08.104
URL / URN: http://dx.doi.org/10.1016/j.ijheatmasstransfer.2013.08.104
Kurzbeschreibung (Abstract):

The influence of intra-droplet heat and mass transfer limitations during the evaporation of binary hydro- carbon mixtures is investigated. Liquid transport processes are described with a 1D formulation (diffu- sion limit model – DLM) taking into account temporal and spatial gradients of the substance properties. The vapor liquid equilibrium is described with a c – u model and the activity coefficients are calculated using the NRTL approach. A suitably normalized segregation factor for each component based on the time-integrated evaporation rate is introduced and used for the analysis of n-heptane/n- decane and n-heptane/iso-octane droplets varying the ambient conditions and the initial liquid compo- sitions. Simulations with the DLM approach are compared to results obtained with a 0D model (rapid mixing model – RMM), which assumes homogeneous droplets in the infinite-diffusivity limit. Simulation results are also compared to experimental data where available. Biot numbers for heat and mass transfer as well as Lewis numbers for the liquid phase are evaluated and their differences are analyzed. A constant Lewis number based approach to calculate the liquid diffusion coefficients is investigated in detail as an alternative to the computationally expensive calculation of the individual diffusion coefficients at each inner droplet location. A suitable strategy to precompute the Lewis number as a function of temperature and composition is presented and the results are compared to the detailed calculations.

Freie Schlagworte: Multicomponent droplet evaporation
Fachbereich(e)/-gebiet(e): 16 Fachbereich Maschinenbau > Fachgebiet Simulation reaktiver Thermo-Fluid Systeme (STFS)
16 Fachbereich Maschinenbau
Hinterlegungsdatum: 03 Nov 2017 07:42
Letzte Änderung: 20 Nov 2017 09:18
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