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Synthesis and high-temperature creep behavior of a SiLuOC-based glass-ceramic

Stabler, Christina ; Seemüller, Christoph ; Choudhary, Ahmad ; Heilmaier, Martin ; Lauterbach, Stefan ; Kleebe, Hans-Joachim ; Ionescu, Emanuel (2016)
Synthesis and high-temperature creep behavior of a SiLuOC-based glass-ceramic.
In: Journal of the Ceramic Society of Japan, 124 (10)
doi: 10.2109/jcersj2.16101
Artikel, Bibliographie

Kurzbeschreibung (Abstract)

In this work, a lutetium-modified silicon oxycarbide (SiOC) glass ceramic was prepared from a single-source precursor via pyrolysis and subsequent hot pressing. It is shown that the main crystalline phase in the hot-pressed SiLuOC is Lu2Si2O7. The high-temperature (HT) creep behavior of SiLuOC was assessed by compression creep experiments performed between 1100 and 1300°C at constant true stresses between 25 and 75 MPa. The calculated viscosity values of SiLuOC were found to be significantly higher as compared to those of SiRE(Al,Mg)ON glasses (RE = rare earth elements). Thus, the presented SiLuOC-based glasses might be used as alternative sintering aids for the liquid-phase sintering of HT creep resistant Si3N4 monolithic samples.

Typ des Eintrags: Artikel
Erschienen: 2016
Autor(en): Stabler, Christina ; Seemüller, Christoph ; Choudhary, Ahmad ; Heilmaier, Martin ; Lauterbach, Stefan ; Kleebe, Hans-Joachim ; Ionescu, Emanuel
Art des Eintrags: Bibliographie
Titel: Synthesis and high-temperature creep behavior of a SiLuOC-based glass-ceramic
Sprache: Englisch
Publikationsjahr: 1 Oktober 2016
Verlag: The Ceramic Society of Japan
Titel der Zeitschrift, Zeitung oder Schriftenreihe: Journal of the Ceramic Society of Japan
Jahrgang/Volume einer Zeitschrift: 124
(Heft-)Nummer: 10
DOI: 10.2109/jcersj2.16101
URL / URN: https://www.jstage.jst.go.jp/article/jcersj2/124/10/124_1610...
Kurzbeschreibung (Abstract):

In this work, a lutetium-modified silicon oxycarbide (SiOC) glass ceramic was prepared from a single-source precursor via pyrolysis and subsequent hot pressing. It is shown that the main crystalline phase in the hot-pressed SiLuOC is Lu2Si2O7. The high-temperature (HT) creep behavior of SiLuOC was assessed by compression creep experiments performed between 1100 and 1300°C at constant true stresses between 25 and 75 MPa. The calculated viscosity values of SiLuOC were found to be significantly higher as compared to those of SiRE(Al,Mg)ON glasses (RE = rare earth elements). Thus, the presented SiLuOC-based glasses might be used as alternative sintering aids for the liquid-phase sintering of HT creep resistant Si3N4 monolithic samples.

Freie Schlagworte: Silicon oxycarbides, SiLuOC glass ceramics, High-temperature creep behavior, Polymer-derived ceramics
Fachbereich(e)/-gebiet(e): 11 Fachbereich Material- und Geowissenschaften
11 Fachbereich Material- und Geowissenschaften > Geowissenschaften
11 Fachbereich Material- und Geowissenschaften > Geowissenschaften > Fachgebiet Geomaterialwissenschaft
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft
11 Fachbereich Material- und Geowissenschaften > Materialwissenschaft > Fachgebiet Disperse Feststoffe
Hinterlegungsdatum: 04 Jan 2017 09:04
Letzte Änderung: 18 Aug 2021 09:53
PPN:
Sponsoren: The German Science Foundation (Deutsche Forschungsgemeinschaft, Bonn, Germany) is gratefully acknowledged for financial support (HE 1872 / 30-1 and IO 64 / 7-1).
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